Isotopic enrichment process
By using the exchange reaction of H2O-H2SiF6·nSiF4 aqueous solution and SiF4 gas in the isotope exchange reaction method, the problems of poor stability and high cost during the silicon isotope concentration process are solved, and low-cost, large-scale isotope concentration and single-unit silicon with excellent thermal conductivity are achieved. Crystalline silicon preparation.
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Embodiment 1
[0091] In this example, use image 3 The shown isotope enrichment device separates and concentrates Si isotopes. As the exchange reaction tower, use the exchange reaction tower that inner diameter 16mm, height 3000mm make exchange reaction tower 2 (the first exchange reaction tower 22 and the 2nd exchange reaction tower 22 ') configuration of fluorine resin exchange reaction tower. A fluororesin-made Rasig ring with an outer diameter of 6 mm was installed inside each exchange reaction column so that the filling height became 2500 mm. In addition, the gas absorption tower 34, the gas generation tower 27, and the gas scrubber 31 use fluororesin columns with an inner diameter of 25mm, which are the same as those used in the exchange reaction tower, and the filling heights of the Lacey rings are 600mm, 400mm, and 800mm, respectively.
[0092] First, 998.8 g of 18.9% by weight hydrofluoric acid is added to the gas absorption tower 34, and while circulating and cooling through the ...
Embodiment 2
[0098] In this example, instead of image 3 The first exchange reaction tower 22 and the second exchange reaction tower 22' of the shown isotope enrichment device use the first exchange reaction tower 41 to the eighth exchange reaction tower 48 made of fluororesin arranged in series to carry out the same process as in Example 1. The same experiment (refer to Figure 4). Each exchange reaction tower has an inner diameter of 25mm and a height of 3000mm. In addition, inside each exchange reaction tower, a fluororesin-made Rasig ring having an outer diameter of 6 mm was set to a filling height of 2500 mm. That is, the total filling height is 20m.
[0099] As a raw material, free hydrofluoric acid containing a concentration of 2.75% by weight and a high silica fluorosilicic acid (H 2 SiF 6 ·SiF 4 ) of high silica fluorosilicic acid aqueous solution. This high-silica fluorosilicic acid aqueous solution is charged into the bottoms of the first exchange reaction tower 41 to the s...
Embodiment 3
[0108] The operable composition range of saturated high silica fluorosilicic acid aqueous solution in Si isotope enrichment operation by gas-liquid contact was investigated. Hydrofluoric acid having a predetermined concentration is allowed to absorb silicon tetrafluoride gas until it becomes saturated, and the composition analysis of the saturated high silica fluorosilicic acid aqueous solution is performed. The concentration of hydrofluoric acid was 10% by weight, 15% by weight, 20% by weight, 25% by weight, 30% by weight, 35% by weight, and 40% by weight. Silicon tetrafluoride was absorbed in a closed system at 0.05 MPaG while cooling the fluororesin container to which 15.0 g of hydrofluoric acid of each concentration was added from the outside with ice water. Usually, at the beginning of absorption, the temperature of the absorption liquid rises due to heat release due to the heat of absorption, and when the saturated concentration is reached, the temperature of the absorpt...
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Abstract
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