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Lithium ion battery anode material and lithium ion battery adopting the lithium ion battery anode material

A technology for lithium-ion batteries and positive electrode materials, applied in battery electrodes, non-aqueous electrolyte battery electrodes, secondary batteries, etc., can solve the problems of large gas production, poor application performance, and high expansion rate

Inactive Publication Date: 2011-11-23
山西襄矿集团中烨能源投资有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0007] Aiming at the problems of poor application performance of cathode materials for nickel-containing lithium-ion batteries, large gas production and high expansion rate in high-temperature environments

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment

[0036] The present invention will be described in detail below based on specific test results.

[0037] The nickel-containing precursor and lithium carbonate were mixed and sintered at 850°C for 24 hours in an air atmosphere, and then pulverized with a mortar to make an active material for positive electrodes.

[0038] Copper foil is used as the current collector of the negative electrode, aluminum foil is used as the current collector of the positive electrode, the sintered lithium cobaltate is used as the positive electrode active material, and MCMB is used as the negative electrode active material. The battery model is square 633770. Lithium cobaltate was mixed with 5% binder PVDF and 4% conductive carbon black, and added to N-methylpyrrolidone at a ratio of 1:1. The negative electrode material can be directly mixed with 10% binder PVDF and added in a ratio of 1:1 to make a slurry. The reconciled positive electrode slurry is coated on the positive electrode current collec...

Embodiment 1

[0044] A plurality of lithium-ion batteries of 633770 squares are made according to the above method, and the median diameter of the battery active material is greater than 6 microns, and the single particle in the primary particle forming secondary spherical particles is analyzed from the electron microscope image The proportion of the total individual particles whose size is above 1 micron is greater than 18%. The battery expansion rate of the fabricated battery is 7.8% under the high temperature storage condition of 85 degrees for 4 hours.

[0045] A plurality of lithium-ion batteries of 633770 square shape are manufactured according to the above-mentioned method, and the content of cobalt and nickel content of the battery active material used are 40% and 13%. The pH value of the positive electrode material used is 11.3. The battery expansion rate of the fabricated battery is 19.8% under the high temperature storage condition of 85 degrees for 4 hours.

Embodiment 2

[0047] A plurality of lithium-ion batteries of 633770 squares are made according to the above method, and the battery active material used is LiNi 0.4 co 0.2 mn 0.4 o 2 The median diameter of its particle size is greater than 6 microns, and the proportion of single particles with a size of more than 1 micron in the primary particles forming secondary spherical particles is greater than 18% in the total single particles. The battery expansion rate of the fabricated battery is 6.7% under the high temperature storage condition of 85 degrees for 4 hours.

[0048] The above experimental results show that, for lithium-ion battery positive electrode materials containing more than 23% nickel content, the particle morphology is secondary spherical large particles of positive electrode materials formed by primary small particles when forming secondary particles When the proportion of particles smaller than 1 micron in the primary particles is greater than 15% of the total primary par...

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Abstract

The invention provides a lithium ion battery anode material of which high temperature performances are stable. The material contains above 23% of nickel. A scanning electron microscope (SEM) graph shows that the material has secondarily spheroidally-shaped microscopic particle morphology, wherein a secondary spheroidal shape is formed through a primary particle agglomeration process, and through control of sizes of primary particles for forming the secondary spheroidal shape, a lithium ion battery anode material of which high temperature performances are stable is obtained. The invention also provides a lithium ion battery adopting the lithium ion battery anode material. The lithium ion battery has the characteristics of high volume specific energy, good high temperature performances and the like.

Description

technical field [0001] The utility model relates to a positive electrode material for a lithium ion battery and a lithium ion battery made of the positive electrode material. Background technique [0002] Since lithium-ion batteries were commercialized in 1991, the cathode materials used in them have also been continuously improved. From the earliest lithium cobalt oxide and lithium manganese oxide to the current multi-element materials, it pursues the continuous improvement of capacity and energy. For the positive electrode material for lithium-ion batteries, lithium nickelate has a relatively high energy density when the charging limit voltage is 4.2V. For example, the invention patent (patent document with application number 200710090083.8) applied by Matsushita Industrial Co., Ltd. in China discloses a positive electrode active material for secondary batteries based on non-aqueous electrolytes and a high-safety non-aqueous electrolyte-based A secondary battery in which...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): H01M4/13H01M10/0525H01M4/131H01M10/0564
CPCY02E60/122Y02E60/12Y02E60/10
Inventor 孙杰蔡松珊
Owner 山西襄矿集团中烨能源投资有限公司