Processes for upgrading algae oils and products thereof
A technology of oil quality and mixture, applied in the petroleum industry, fat oil/fat production, refined hydrocarbon oil, etc.
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Embodiment 1
[0113] The algal oil feedstock was produced from Nannochloropsis algae by hydrothermal treatment and heptane extraction according to the method outlined in the previous section "Hydrothermal Treatment of Biomass and Acidification to Produce Crude Algal Oil". The hydrothermal treatment step (step b in the method listed above) was carried out at 260°C for 0.5 hours. The obtained algal oil feedstock was subjected to various hydroprocessing experiments, including decarboxylation (1SEBR), hydrogenation (2SEBR), decarboxylation followed by hydrogenation (3SEBR) and three catalytic hydrotreatments (4SEBR, 5SEBR and 6SEBR). The algae oil feedstock was also heat treated in hydrogen (no catalyst, 7SEBR). Table 1 summarizes the conditions and reagent pools for these experiments, figure 1 The oil products of these experiments are shown.
[0114] Table 1: Catalyst / Process Conditions
[0115]
[0116] Experimental runs for groups 1-7SEBR were performed in a semi-batch reactor (in the ...
Embodiment 2
[0170] Additional experiments were performed with the same Nannochloropsis-derived algae oil feedstock as in Example 1, but the feedstock was upgraded under different process conditions. Specifically, the effects of increasing reaction temperature, retention time, and hydrogen pressure on algal oil upgrading were investigated. According to the aforementioned procedure of the present invention, elemental analysis (EA) and high temperature GC-MS analysis were performed on the produced algae oil products and samples.
[0171] Table 8 lists the run samples and corresponding experimental conditions. Thus, the run samples of this example included a higher decarboxylation test temperature (375°C) than the decarboxylation run 1SEBR (350°C). Therefore, the results of running 1SEBR and 8SEBR were compared, as shown in Table 8. Run 9SEBR was catalytic hydrotreating at 1000 psig, but the retention time (2 hours) was longer than the catalytic hydrotreating run in Example 1 (1 hour), ther...
Embodiment 3
[0184] Using the same algal oil feedstock derived from Nannochloropsis as in Example 1, additional experiments were performed by catalytic cracking of the algal oil feedstock in a Micro Catalytic Cracking (MAT) system. MAT equipment and testing are well known in petroleum processing R&D and have been designed and developed over the years to be highly consistent with large fluid catalytic cracking (FCC) units.
[0185] The predictive power of the MAT test is quite remarkable considering that only gram-scale feedstock is required, while commercial FCC units can process feedstock in excess of 1 million barrels per day (MBPD). Like commercial FCC units, the MAT test operates at cracking temperatures of about 1000 degrees Fahrenheit, with very short catalyst-feedstock contact times (5-10 seconds), and uses zeolite-based catalysts at atmospheric pressure.
[0186] In the present embodiment, the MAT test is used to compare the FCC process and the
[0187] A reference petroleum feeds...
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Abstract
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