Modified resins and resin compositions
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Embodiment 1
[0609] Adipic acid dihydrazide and polyisocyanate (DURANATE TPA-100, manufactured by Asahi Kasei Chemical Co., Ltd.) were charged so that the equivalent ratio of isocyanate group to hydrazide group was 1.0, and butyl acetate was mixed to prepare a dispersion with a solid content of 10%. . The dispersion was stirred at 120° C. for 12 hours. Collect a part of the reaction solution with 1 As a result of H-NMR analysis, the peak around 3.3 ppm derived from isocyanate disappeared. After butyl acetate was distilled off with a rotary evaporator, heat resistance was evaluated. The evaluation results are listed in Table 1.
Embodiment 2
[0611] 36 g of hydrazine monohydrate was dissolved in 1 L of isopropanol, cooled to 0° C., and 50 g of hexamethylene diisothiocyanate was added while stirring. The resulting solids are recovered by filtration for use in 1 H-NMR was analyzed, and the result was 4,4'-hexamethylenebisthiosemicarbazide.
[0612] For this 4,4'-hexamethylenebisthiosemicarbazide and polyisocyanate (DURANATE TPA-100, manufactured by Asahi Kasei Chemical Co., Ltd.), the same method as in Example 1 was carried out to evaluate heat resistance. The evaluation results are listed in Table 1.
Embodiment 3
[0614] 36 g of hydrazine monohydrate was dissolved in 1 L of isopropanol, cooled to 0° C., and 50 g of hexamethylene diisocyanate was added while stirring. The resulting solids are recovered by filtration for use in 1 H-NMR is analyzed, and the result is 4,4'-hexamethylenebisemicarbazide.
[0615] For this 4,4'-hexamethylene bisaminocarbazide and polyisocyanate (DURANATE TPA-100, manufactured by Asahi Kasei Chemical Co., Ltd.), the same method as in Example 1 was carried out to evaluate heat resistance. The evaluation results are listed in Table 1.
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