Micro-nano tungsten/molybdenum/tantalum carbide solid-solution composite powder and preparation method thereof
A technology of composite powder and tungsten carbide, which is applied in the field of powder metallurgy, can solve the problems of affecting the structure of ceramic body, heavy metal segregation, failure to achieve solid solution strengthening, etc., and achieve the effect of uniform distribution
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Embodiment 1
[0028] (1) Ingredients: Weigh 850g of tungsten powder, 420g of molybdenum powder, 420g of tantalum powder and 150g of graphite powder, and add 75g of cerium oxide powder; the purity of tungsten powder, molybdenum powder, tantalum powder and graphite powder is >99.9%, and the average particle size 20~100μm; the average particle size of cerium oxide powder is less than 20μm;
[0029] (2) High-energy ball milling solid phase reaction: Put the raw materials prepared in step (1) together with tungsten carbide balls into a stainless steel vacuum ball mill tank for high-energy ball milling. The ball-material ratio is 10:1, and the ball milling speed is 300 rpm. The time is 36h, and the mixed powder of (Mo, Ta)C solid solution powder and W+C+(W, Mo, Ta)C is obtained;
[0030] (3) Thermal combination reaction: put the reaction product obtained in step (2) into a high-temperature atmosphere furnace, and carry out a thermal combination reaction at 800°C for 60 minutes in a nitrogen-hydro...
Embodiment 2
[0033] (1) Ingredients: Weigh 1050g of tungsten powder, 410g of molybdenum powder, 510g of tantalum powder and 130g of graphite powder, and add 90g of cerium oxide powder; the purity of tungsten powder, molybdenum powder, tantalum powder and graphite powder is >99.9%, and the average particle size 20~100μm; the average particle size of cerium oxide powder is less than 20μm;
[0034] (2) High-energy ball milling solid phase reaction: Put the raw materials prepared in step (1) together with tungsten carbide balls into a stainless steel vacuum ball mill tank for high-energy ball milling. The ball-material ratio is 6:1, and the ball milling speed is 200 rpm. The time is 24h to obtain (Mo, Ta)C solid solution powder and W+C+(W, Mo, Ta)C mixed powder;
[0035] (3) Thermal combination reaction: put the reaction product obtained in step (2) into a high-temperature atmosphere furnace, and carry out a thermal combination reaction at 900°C for 120 minutes under a nitrogen-hydrogen mixed ...
Embodiment 3
[0037] (1) Ingredients: Weigh 1150g of tungsten powder, 360g of molybdenum powder, 450g of tantalum powder and 140g of graphite powder, and add 90g of cerium oxide powder; the purity of tungsten powder, molybdenum powder, tantalum powder and graphite powder is >99.9%, and the average particle size 20~100μm; the average particle size of cerium oxide powder is less than 20μm;
[0038] (2) High-energy ball milling solid phase reaction: Put the raw materials prepared in step (1) together with tungsten carbide balls into a stainless steel vacuum ball milling tank for high-energy ball milling. The ball-material ratio is 9:1, and the ball milling speed is 300 rpm. The time is 36h, and the mixed powder of (Mo, Ta)C solid solution powder and W+C+(W, Mo, Ta)C is obtained;
[0039](3) Thermal combination reaction: put the reaction product obtained in step (2) into a high-temperature atmosphere furnace, and carry out a thermal combination reaction at 850°C for 90 minutes in a nitrogen-hyd...
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