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Method for preparing polylactic acid composite material by modifying papermaking white mud

A technology for papermaking lime mud and composite materials, which is applied in the field of preparing polylactic acid composite materials by modification of papermaking lime mud, can solve problems such as environmental pollution and resource waste, and achieve the effect of solving resource waste and realizing sustainable recycling.

Inactive Publication Date: 2016-04-20
常州市鼎升环保科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The invention not only solves the problems of resource waste and environmental pollution, but also realizes the sustainable recycling of resources, and the obtained polylactic acid composite material has good heat resistance and impact resistance

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0017] First collect papermaking white mud, mix it with 1mol / L hydrochloric acid solution according to the solid-to-liquid mass ratio of 1:10, and place it under 200W for 10 minutes of ultrasonic oscillation, then soak for 2 hours, and filter it after soaking is completed. Collect the filter cake, and then according to the solid-liquid mass ratio of 1:10, stir and mix the filter cake with 20% sodium hydroxide solution and let it settle, filter and collect the filter cake again, wash with deionized water until the pH reaches 7.0 , and placed in a 60°C oven to dry for 6 hours to obtain the washed and dried lime mud; then put the washed and dried lime mud in a tube furnace and heat it, setting the heating rate to 10°C / min. When the temperature rises to 200°C, stop heating. After heat preservation and calcination for 3 hours, slowly heat up to 400°C at a rate of 2°C / min, then calcine at a constant temperature for 2 hours, then slowly heat up to 600°C at a rate of 10°C / min, and heat...

example 2

[0020]First collect papermaking white mud, mix it with 1mol / L hydrochloric acid solution according to the solid-to-liquid mass ratio of 1:10, and place it under 250W for 13 minutes of ultrasonic oscillation, then soak it for 2.5 hours, and filter it after soaking , collect the filter cake, and then according to the solid-to-liquid mass ratio of 1:10, the filter cake and the sodium hydroxide solution with a mass concentration of 20% are stirred and mixed and allowed to stand for precipitation, and the filter cake is collected again by filtration, washed with deionized water until the pH is up to 7.0, and placed in a 70°C oven to dry for 7 hours to obtain the washed and dried lime mud; then place the washed and dried lime mud in a tube furnace and heat it, setting the heating rate to 10°C / min, When the temperature rises to 225°C, stop heating. After 4 hours of heat preservation and calcination, slowly raise the temperature to 425°C at a rate of 2°C / min, then calcine at a constant...

example 3

[0023] First collect papermaking white mud, mix it with 1mol / L hydrochloric acid solution according to the solid-to-liquid mass ratio of 1:10, and place it under 300W for ultrasonic oscillation for 15 minutes, then soak for 3 hours, and filter it after soaking is completed. Collect the filter cake, and then according to the solid-liquid mass ratio of 1:10, stir and mix the filter cake with 20% sodium hydroxide solution and let it settle, filter and collect the filter cake again, wash with deionized water until the pH reaches 7.0 , and placed in an oven at 80°C for 8 hours to obtain washed and dried lime mud; then put the washed and dried lime mud in a tube furnace and heat it, setting the heating rate to 10°C / min, and then When the temperature rises to 250°C, stop heating. After heat preservation and calcination for 5 hours, slowly heat up to 450°C at a rate of 2°C / min, then calcine at a constant temperature for 3 hours, then slowly heat up to 650°C at a rate of 10°C / min, and h...

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Abstract

The invention discloses a method for preparing a polylactic acid composite material by modifying papermaking white mud, and belongs to the field of resource reutilization. The method comprises the following steps: collecting papermaking white mud, mixing the papermaking white mud with hydrochloric acid and a sodium hydroxide solution, filtering the mixture to obtain filter cakes, performing heat preservation calcining and carbonization on the filter cakes, grinding the processed filter cakes into grains, adding 3-aminopropyltriethoxysilane and absolute ethyl alcohol to the grains, ultrasonically oscillating the grains, performing plasma radio frequency modification, compounding the modified grains with polylactic acid grains, extruding, pelletizing and drying the compound to prepare the polylactic acid composite material. The method for preparing the polylactic acid composite material by modifying the papermaking white mud has the following benefits: the problems of resource waste and environment pollution are solved, and sustainable cyclic utilization of the resource is achieved; the prepared polylactic acid composite material has good heat resistance and impact resistance, can resist the temperature of 105-120 DEG C and has the shock strength of 15-17 KJ / m2 and the tensile elongation at break of 50-55%.

Description

technical field [0001] The invention relates to a method for preparing a polylactic acid composite material by modifying papermaking white mud, and belongs to the field of resource reuse. Background technique [0002] Pulp and paper mills will produce a large amount of causticized lime mud during the alkali recovery process, also known as papermaking lime mud, which uses wood as raw material. Some large paper mills abroad and at home use lime kiln calcination method to make The lime mud is regenerated to produce recycled lime, which is recycled in causticization. However, for pulp and paper enterprises that use non-wood fibers as raw materials, due to the high silicon content of white mud, recycling and recycling will aggravate the silicon interference of alkali recovery, so that alkali recovery cannot operate normally, and white mud cannot be properly treated. The use of filling pits to pave roads or direct discharge into rivers not only causes waste of resources and envir...

Claims

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Application Information

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IPC IPC(8): C08L67/04C08K9/02C08K9/06C08K9/00C08K3/22C08K3/26
CPCC08K9/02C08K3/22C08K3/26C08K9/00C08K9/06C08K2003/2206C08K2003/265C08L2201/08C08L67/04
Inventor 许斌盛艳花高力群
Owner 常州市鼎升环保科技有限公司