Reverse osmosis membrane and preparation method and application thereof
A technology of reverse osmosis membrane and reaction time, applied in the field of reverse osmosis membrane, preparation, and sulfonated polyamide composite reverse osmosis membrane, can solve the problems of unattainable performance, high salt rejection, unable to get rid of the constraints of MPD chemical structure, etc. The effect of excellent durability, simple synthesis process and easy promotion
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Embodiment 1
[0038] Embodiment 1N, the synthesis of N'-di(4-sulfophenyl)methylenediamineN,N'-bis(4-sulfophenyl)methyldiamine (NSMDA), its structural formula is:
[0039]
[0040] (1) Synthesis of A
[0041] Put 28.6g of benzotriazole white flocculent powder and 250mL of ethanol in a 500mL round-bottomed flask, slowly add 22.5g of aniline solution and 7mL of formaldehyde solution, fix it on an iron stand, stir at room temperature, obtain a white precipitate after 8 hours, pump After filtering and washing with ethanol, 28.6 g of white solid A was obtained (the yield was about 75%).
[0042] (2) Synthesis of B
[0043] Put 28.6gA in a 500mL round bottom flask, add 200mL tetrahydrofuran solution, then slowly add 11.0g sodium borohydride, install a reflux condenser at the mouth of the bottle, and place it in an oil bath for 60 o C was stirred and refluxed, and a viscous liquid was obtained after 12 hours. After suspension steaming, water was added, and dilute hydrochloric acid was added to...
Embodiment 2
[0051] Embodiment 2N, the synthesis of N'-di(4-sulfophenyl)ethylenediamineN,N'-bis(4-sulfophenyl)ethylenediamine (NSEDA), whose structural formula is:
[0052]
[0053] (1) Synthesis of A
[0054] Put 28.6g of benzotriazole white flocculent powder and 250mL of ethanol in a 500mL round-bottomed flask, slowly add 22.5g of aniline solution and 14mL of glyoxal solution, fix it on an iron stand, stir at room temperature, and obtain a white precipitate after 8 hours , and washed with ethanol after suction filtration to obtain white solid A42.1g (yield about 80%).
[0055] (2) Synthesis of B
[0056] Put 32.1gA in a 500mL round bottom flask, add 200mL tetrahydrofuran solution, then slowly add 11.0g sodium borohydride, install a reflux condenser at the mouth of the bottle, place in an oil bath for 60 o C was stirred and refluxed. After 12 hours, a viscous liquid was obtained. After suspension steaming, water was added, and dilute hydrochloric acid was added to adjust the pH to 3-...
Embodiment 3
[0064] Embodiment 3N, the synthesis of N'-di(4-sulfophenyl)propylenediamineN,N'-bis(4-sulfophenyl)propylenediamine (NSPDA), whose structural formula is:
[0065]
[0066] (1) Synthesis of A
[0067] Put 28.6g of benzotriazole white flocculent powder and 250mL of ethanol in a 500mL round-bottomed flask, slowly add 22.5g of aniline solution and 16mL of methylglyoxal solution, fix it on an iron stand, stir at room temperature, and obtain a white precipitate after 8 hours. After suction filtration and washing with ethanol, 48.4 g of white solid A was obtained (the yield was about 83%).
[0068] (2) Synthesis of B
[0069] Put 33.8gA in a 500mL round bottom flask, add 200mL tetrahydrofuran solution, then slowly add 11.0g sodium borohydride, install a reflux condenser at the mouth of the bottle, place in an oil bath for 60 o C was stirred and refluxed, and a viscous liquid was obtained after 12 hours. After suspension steaming, water was added, and dilute hydrochloric acid was ...
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