The application discloses a high-flux
fiber physiological
electrode, a preparation method, an
electrode array and application thereof, and belongs to the field of
flexible electronics and biomedical sensing. The
electrode adopts a three-layer coaxial
fiber structure, the inner layer is a high-
conductivity core layer containing MXene, carbon nanotubes and poly 3,4-ethylenedioxythiophene, the middle layer is an insulating layer such as
polydimethylsiloxane, and the outer layer is a self-
adhesive layer based on dynamic bond cross-linked
polyvinyl alcohol and
polyacrylic acid. The
diameter of a
single fiber is 50-100 mu m. By utilizing the reversible adhesion characteristics of the outer layer dynamic bond and / or non-
covalent interaction, multiple fibers can be freely assembled into a high-density and reconfigurable
electrode array. The array has excellent electrochemical performance, mechanical matching, interface adhesion stability and
biocompatibility, and has a stimulation response and self-healing ability, is suitable for long-term stable wearable
physiological monitoring and implantable closed-loop neural interface, and can realize high
spatiotemporal resolution bioelectric
signal recording and regulation.