A coating composition and a method of imparting a self-healing property and other properties onto a substrate
A composition and coating technology, applied in the direction of cyclodextrin coatings, zinc organic compounds, tin organic compounds, etc., can solve the problems of exposure to ultraviolet light, carbon dioxide, water or other external sources
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example 1
[0032] According to one embodiment of the present invention, the polymer (PCL-HDI) network is prepared by in situ polymerization of hexamethylene diisocyanate trimer (HDI) and polycaprolactone diol (PCL diol). The polymerization is carried out in the presence of bismuth neodecanoate or triethylamine catalysts. The polymer network is elastic and imparts self-healing properties to coatings formed from the coating compositions of the present invention. The polymer network is composed of HDI hard segment and PCL diol soft segment. Figure 2a The synthesis of a PCL diol-HDL polymer network according to one embodiment of the invention is shown. Figure 3a and 3b ATR-FTIR spectra of PCL diol-HDI polymer films in the presence of two different catalysts are shown. In this example, the isocyanate groups in the HDI react with the OH groups in the PCL diol to form urethane linkages, thereby forming a polyurethane network with hydrogen bonds for self-healing. Molar ratios of isocyanate...
example 2
[0035] According to one embodiment of the invention, the polymer (PCL triol-HDI) network is prepared by in situ polymerization of hexamethylene diisocyanate trimer and polycaprolactone triol. The polymerization is carried out in the presence of bismuth neodecanoate. The polymer network is elastic and imparts self-healing properties to coatings formed from the coating compositions of the present invention. The polymer network is composed of HDI hard segment and PCL triol soft segment.
example 3
[0037] The polymer network according to another embodiment of the present invention is composed of a polyurethane backbone formed by HDI and PEG and cyclodextrin as side chains. The cyclodextrin ring was introduced into PEG, and the -NCO group of HDI reacted with the -OH group of PEG in the presence of an organotin catalyst. Figure 4 A synthetic scheme for the HDI-PEG-cyclodextrin polymer network is shown. Figure 5 is the ATR-FTIR spectrum of HDI-PEG-cyclodextrin polymer. The self-healing ability is achieved through hydrogen bonding of the polyurethane backbone and the sliding and movement of cyclodextrin rings along the polyurethane chain.
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