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A kind of amidoximated composite fiber and preparation method thereof

A composite fiber and fiber technology, applied in chemical instruments and methods, alkali metal compounds, inorganic chemistry, etc., can solve the problems of high manufacturing cost, low adsorption capacity, poor adsorption selectivity, etc.

Active Publication Date: 2021-06-15
CGN DASHENG ELECTRON ACCELERATOR TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, these adsorbents generally have problems such as high manufacturing cost, low adsorption capacity, and poor adsorption selectivity.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0024] The invention provides a kind of preparation method of amidoximation composite fiber, comprises the following steps:

[0025] a) dissolving polyvinyl alcohol and polyacrylonitrile in a solvent to obtain a stock solution;

[0026] b) performing defoaming, spinning and coagulation molding on the stock solution to obtain composite fibers;

[0027] c) placing the composite fiber in an aqueous solution of acrylonitrile, and performing electron beam irradiation treatment to obtain an irradiated fiber;

[0028] d) heat-treating the irradiated fibers in an aqueous solution of hydroxylamine hydrochloride to obtain amidoximated composite fibers.

[0029] In the present invention, specific polyvinyl alcohol and polyacrylonitrile are spun to obtain composite fibers, and then electron beam irradiation treatment is carried out in a specific acrylonitrile solution to cross-link the composite fibers and improve the strength of the fibers themselves. At the same time, the acrylic Nitr...

Embodiment 1

[0051] Polyvinyl alcohol and polyacrylonitrile were dissolved in dimethyl sulfoxide at 80° C. at a mass ratio of 90:10 to obtain a stock solution with a solid content of 10%. The stock solution is defoamed (temperature is 80°C, air pressure is 1 / 4 atmospheric pressure), spinning (temperature is 90°C), solidified and formed (sodium sulfate-sulfuric acid coagulation bath, temperature is 45°C), and then heat-stretched (the temperature is 180° C., and the draw ratio is 4 times), heat setting treatment (the temperature is 180° C., and the duration is 3 minutes), to obtain a composite fiber.

[0052] The obtained composite fiber is placed in an acrylonitrile aqueous solution with a mass concentration of 9%, and irradiated with an electron beam of 10kGy; then it is taken out and cleaned, and then placed in an aqueous solution of hydroxylamine hydrochloride with a mass concentration of 25%, and the hydroxylamine hydrochloride in the aqueous solution of hydroxylamine hydrochloride and ...

Embodiment 2

[0054] Polyvinyl alcohol and polyacrylonitrile were dissolved in dimethyl sulfoxide at 80° C. at a mass ratio of 90:10 to obtain a stock solution with a solid content of 10%. The stock solution is defoamed (temperature is 80°C, air pressure is 1 / 4 atmospheric pressure), spinning (temperature is 90°C), solidified and formed (sodium sulfate-sulfuric acid coagulation bath, temperature is 45°C), and then heat-stretched (the temperature is 180° C., and the draw ratio is 4 times), heat setting treatment (the temperature is 180° C., and the duration is 3 minutes), to obtain a composite fiber.

[0055] The obtained composite fiber is placed in an acrylonitrile aqueous solution with a mass concentration of 9%, and irradiated with an electron beam of 20kGy; then it is taken out and cleaned, and then placed in an aqueous solution of hydroxylamine hydrochloride with a mass concentration of 25%, and the hydroxylamine hydrochloride in the aqueous solution of hydroxylamine hydrochloride and ...

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Abstract

The invention provides an amidoximated composite fiber and a preparation method thereof. The preparation method provided by the present invention includes: a) dissolving polyvinyl alcohol and polyacrylonitrile in a solvent to obtain a stock solution; b) degassing, spinning and solidifying the stock solution to obtain a composite fiber; c) dissolving the The composite fiber is placed in an acrylonitrile aqueous solution, and subjected to electron beam irradiation treatment to obtain an irradiated fiber; d) heat-treating the irradiated fiber in an aqueous solution of hydroxylamine hydrochloride to obtain an amidoximated composite fiber. According to the preparation method of the present invention, acrylonitrile molecules are firstly grafted onto the fibers, and then amidoxime groups of small molecular weight are grafted on the fibers to obtain amidoximated composite fibers. The fiber can be used for uranium extraction in seawater and has high adsorption capacity for uranyl ions.

Description

technical field [0001] The invention relates to the technical field of adsorption materials, in particular to an amidoximated composite fiber and a preparation method thereof. Background technique [0002] Uranium is an important raw material for nuclear power, and the development of uranium resources is an important demand for the development of nuclear power in my country. However, my country's land uranium resources are scarce, and seawater is a shared resource. The total amount of uranium resources is 4.5 billion tons, which is equivalent to 1000% of the uranium content in land ores. times. Therefore, uranium resources in seawater are a promising source of nuclear fuel supply and an inevitable trend in the development of the nuclear industry in the future. It is of great significance to extract uranium resources in seawater. [0003] Uranium resources mainly exist in the form of uranyl ions in the ocean. Since the 1960s, Japan, the United States, France and other countr...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/26B01J20/28B01J20/30
CPCB01J20/265B01J20/28023
Inventor 王千宇苏春左都文邵晓沈屹立
Owner CGN DASHENG ELECTRON ACCELERATOR TECH