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A kind of preparation method and application of mhpbs-hemin/rgo labeled electrochemical immunosensor

An immunosensor, electrochemical technology, applied in the direction of chemical instruments and methods, electrochemical variables of materials, nanotechnology for sensing, etc., can solve the problems of cumbersome sample pretreatment, long detection cycle, unsatisfactory, etc., and achieve relief Effects of irreversible stacking phenomenon, reduction of aggregation and deactivation, and improvement of sensitivity

Active Publication Date: 2021-03-09
SHANDONG UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] At present, the detection of aflatoxins mainly includes thin film chromatography and liquid chromatography, but these two methods have a long detection cycle, cumbersome sample pretreatment, and complicated operations, which can no longer meet the needs of modern society.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0042] Example 1 A method of preparing an electrochemical immunosensor of MHPBS-HEMIN / RGO, steps are as follows:

[0043] (1) Polishing a glass carbon electrode having a diameter of 4.0 mm into a mirror surface, and clean it in ultrapure water;

[0044] (2) Take 6.0 μL of MUA-Au NPS to the surface of the electrode, dry at room temperature, clean the surface of the electrode with ultrapure water, dry;

[0045] (3) Continue to capture antibody ABs from 6.0 μL, 10.0 μg / ml of yellowlaxin 1 Add to the surface of the electrode, place it in a 4.0 ° C refrigerator;

[0046] (4) 3.0 μL, 0.5% of the bovine serum protein BSA solution is added to the surface of the electrode to enclose the non-specific active site on the surface of the electrode, and the electrode surface is cleaned with phosphate buffer with pH = 7.2, placed in 4.0 °. Ceiling in the C refrigerator;

[0047] (5) A series of different concentrations of a series of different concentrations of a series of xeroxin antigenic s...

Embodiment 2

[0049] Example 2 A method of preparing an electrochemical immunosensor of MHPBS-HEMIN / RGO, steps are as follows:

[0050] (1) Polishing a glass carbon electrode having a diameter of 4.0 mm into a mirror surface, and clean it in ultrapure water;

[0051] (2) Take 6.0 μL of MUA-Au NPS to the surface of the electrode, dry at room temperature, clean the surface of the electrode with ultrapure water, dry;

[0052] (3) Continue to capture antibody ABs from 6.0 μL, 15.0 μg / ml 1 Add to the surface of the electrode, place it in a 4.0 ° C refrigerator;

[0053] (4) 3.0 μL, 1.0% of the bovine serum protein BSA solution is added to the surface of the electrode to enclose the non-specific active site on the surface of the electrode, and the electrode surface is cleaned with phosphate buffer with pH = 7.2, placed in 4.0 °. Ceiling in the C refrigerator;

[0054] (5) Add 6.0 μL, 1.0 pg / ml ~ 100.0 ng / ml of a series of different concentrations of yellowlaxin antigenic solution, after 35.0 ...

Embodiment 3

[0056] Example 3 A method of preparing an electrochemical immunosensor of MHPBS-HEMIN / RGO, steps are as follows:

[0057] (1) Polishing a glass carbon electrode having a diameter of 4.0 mm into a mirror surface, and clean it in ultrapure water;

[0058] (2) Take 6.0 μL of MUA-Au NPS to the surface of the electrode, dry at room temperature, clean the surface of the electrode with ultrapure water, dry;

[0059] (3) Continue to capture antibody ABs from 6.0 μL, 20.0 μg / ml of yellowlaxin 1 Add to the surface of the electrode, place it in a 4.0 ° C refrigerator;

[0060] (4) 3.0 μL, 1.5% bovine serum protein BSA solution is added to the surface of the electrode, and the non-specific active site on the surface of the electrode is to be cleaned with pH = 7.2 phosphate buffer, placed in 4.0 °. Ceiling in the C refrigerator;

[0061] (5) Add 6.0 μL, 1.0 pg / ml ~ 100.0 ng / ml of a series of different concentrations of yellowlaxin antigen solution, 40.0 min in a 4.0 ° C refrigerator, w...

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PUM

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Abstract

The invention belongs to the technical fields of novel nanomaterials, immune analysis and biosensing detection, and provides a preparation method and application of an mHPBs‑Hemin / rGO-labeled electrochemical immunosensor. The present invention introduces the mesoporous hollow Prussian blue nano-cubic spaced hemin functionalized graphene porous composite material as the current signal amplification mechanism into the construction of the electrochemical immunosensor for the first time, and efficiently amplifies the current response signal to realize the detection of aflatoxin Quantitative and sensitive detection. The electrochemical immunosensor of the invention is easy to operate, low in cost, high in sensitivity and wide in detection range, and has important scientific significance and application value for the quantitative and sensitive detection of aflatoxins.

Description

Technical field [0001] The present invention belongs to the novel functional nanomaterial, immunoassay and biosensor detection technology, and provides a method and application of an electrochemical immunosensor of MHPBS-HEMIN / RGO. Background technique [0002] Huangquisin is a very poisonous fungal toxin. As early as 1993, Huangquisin is delineated by the World Health Organization WHO as a kind of carcinogens, which is the first in the current carcinogens. Huangquisin is widely present in grain and oil crops such as corn, wheat, peanuts and various meats, dairy products, have strong destructive organizational organizations such as people and animals, and will inevitably in the production and life. Cancer or even death is caused seriously. According to the national food hygiene standard, corn, peanut, the allowed maximum content of the yellow guisoxin B1 is 20 μg / kg, while the standard of the European Union is 2μg / kg, and the intensive precise detection of Huangquis is impo...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): G01N27/327G01N27/30G01N27/26G01N33/543G01N33/58B01J31/18B01J35/00B01J35/10B82Y15/00B82Y30/00
CPCG01N27/3278G01N27/308G01N27/26G01N33/5438G01N33/54386G01N33/58B01J31/183B82Y15/00B82Y30/00B01J2531/842B01J35/33B01J35/60B01J35/61
Inventor 李月云张春燕禹晓东张栓贾翌雷李新进徐振
Owner SHANDONG UNIV OF TECH