A kind of amphiphilic polymer for surface biofunctionalization and its preparation method and application
A polymer, amphiphilic technology, applied in the field of polymers, can solve the problems of harsh conditions for block copolymerization, restricting block polymers, and difficult to change flexibly, so as to expand different biomedical applications, achieve diversity, and avoid cumbersome and inefficient effects
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[0117] The preparation method of the present invention will be further described in detail below in conjunction with specific examples. It should be understood that the following examples are only for illustrating and explaining the present invention, and should not be construed as limiting the protection scope of the present invention. All technologies realized based on the above contents of the present invention are covered within the scope of protection intended by the present invention.
[0118] Unless otherwise specified, the experimental methods used in the following examples are conventional methods; the reagents and materials used in the following examples, unless otherwise specified, can be obtained from commercial sources.
[0119] The HEPES buffer used in the following examples is a buffer solution with a concentration of 100 mM and a pH of 7.0.
[0120]Optional means that the feature exists or does not exist, and also means that the feature must exist, but the spe...
Embodiment 1
[0121] Example 1 Synthesis of amphiphilic polymer OA25-PLL-PEG2k-NTA30
[0122] Weighed 8.5 mg of poly-L-lysine (PLL, average molecular weight 22,500 Da, purchased from Shanghai Yuanye Company) in a 2 ml centrifuge tube, and dissolved it in 200 μL of HEPES buffer to obtain a solution (1).
[0123] Weigh 24 mg of polyethylene glycol 2000 (NHS-PEG2k-NTA) modified with succinimidyl ester (NHS) and nitrilotriacetic acid (NTA) at both ends respectively, and the average molecular weight of polyethylene glycol is 2000Da, purchased from Nanocs Corporation of the United States. ), which was dissolved in 100 μL N,N-dimethylformamide (analytical grade, Beijing Chemical Plant) to obtain solution (2).
[0124] Measure 3.2 μL of oleic acid (molecular weight 282.5, purchased from Beijing Chemical Plant, purified by distillation) in a glass vial, and place it in 100 μL N,N-dimethylformamide to obtain solution (3).
[0125] Mix the above solution (1), solution (2) and solution (3) in a centri...
Embodiment 2
[0129] Example 2 Synthesis of amphiphilic polymer OA25-PLL-PEG5k-NTA30
[0130] Similar to Example 1, the difference is that 60 mg of polyethylene glycol 5000 (NHS-PEG5k-NTA, polyethylene glycol with an average molecular weight of 5000 Da, purchased from the U.S. Nanocs Company), which was dissolved in 100 μL N,N-dimethylformamide to obtain solution (2). 37 mg of white lyophilized powder were obtained.
[0131] The white powder is a functionalized amphiphilic polymer grafted with 25% oleic acid and 30% polyethylene glycol 5k-nitrilotriacetic acid, and the polymer is named OA25-PLL-PEG5k-NTA30.
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