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Passivation method of sulfuration type hydrogenation catalyst

A hydrogenation catalyst and vulcanization-type technology, applied in the direction of physical/chemical process catalysts, catalyst protection, chemical instruments and methods, etc., can solve problems affecting product quality, recycling refinery troubles, etc., and achieve the effect of avoiding spontaneous reactions

Active Publication Date: 2021-07-16
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The protective film formed by this type of liquid-phase passivator can be removed during the reaction, but the recovery of the removed liquid may bring trouble to the refinery, and it may affect the quality of the product after it is mixed with the raw material oil

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] Take the industrially produced catalyst FH-40C and pre-sulfurize it to make a sulfided catalyst. Put the catalyst in a closed container to evacuate with a vacuum degree of -0.05MPa, then cool down to -180°C and feed nitrogen gas. 100mL / h, keep it for 1h, turn off the nitrogen, raise the temperature to -100°C, introduce nitrogen containing 15% ozone, the gas pressure is 3.5MPa, the flow rate is 1000mL / h, keep it for 0.5h, the finished catalyst A is obtained, and replace it with nitrogen After replacement, the catalyst is taken out for use.

Embodiment 2

[0027] Take the industrially produced catalyst FH-40C and pre-sulfurize it to make a sulfided catalyst, place the catalyst in a closed container to evacuate, the vacuum degree is -0.1MPa, then cool down to -50°C and feed carbon dioxide, the carbon dioxide pressure is 1MPa, the flow rate 200mL / h, keep 2h, turn off the carbon dioxide, raise the temperature to -10°C, introduce carbon dioxide gas containing 10% ozone, gas pressure 4.0MPa, flow rate 1200mL / h, keep 0.2h, then raise the temperature to 20°C, the flow rate is 1500ml / h, keep it for 0.1h to get the finished catalyst B, replace it with nitrogen and take out the catalyst for use.

Embodiment 3

[0029] Take the industrially produced catalyst 1 and pre-sulfurize it to make a sulfided catalyst, place the catalyst in a closed container to evacuate with a vacuum degree of -0.08MPa, then cool down to -160°C and feed nitrogen with a nitrogen pressure of 5MPa and a flow rate of 200mL / h, keep it for 2h, turn off the nitrogen, raise the temperature to -80°C, introduce nitrogen containing 10% ozone, the gas pressure is 6.0MPa, the flow rate is 2000ml / h, keep it for 0.5h, then raise the temperature to -50°C, and increase the flow rate to 3000mL / h, kept for 0.1h, the finished catalyst C was obtained, replaced by nitrogen, and the catalyst was taken out for use.

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Abstract

The invention discloses a passivation method of a sulfuration type hydrogenation catalyst, which comprises the following steps: placing the sulfuration type hydrogenation catalyst in a closed container, vacuumizing and cooling the container, and introducing nitrogen or carbon dioxide for treatment; and heating the obtained material, and finally carrying out passivating treatment by using passivating gas. According to the method, ozone is adopted to passivate the catalyst at low temperature, so that a compact oxide layer is formed on the surface of the catalyst, oxygen in air is prevented from further acting with metal sulfide in a catalyst pore channel, a self-heating reaction of the catalyst is avoided, and the safety of storage, transportation and filling of the catalyst is improved.

Description

technical field [0001] The invention belongs to the technical field of petrochemical industry, and in particular relates to a treatment method of a sulfurized hydrogenation catalyst. Background technique [0002] In recent years, the tendency of crude oil to become inferior has become increasingly obvious, while the demand for clean fuels in various countries is increasing. Hydrogenation process is one of the most effective means of producing clean fuels, and efficient hydrogenation catalysts are the key to this process. Conventional hydrogenation catalysts are in an oxidized state, but the active substances are in a sulfurized state in actual use, so they need to be sulfurized in the reactor before use. At present, the most common ones are internal pre-vulcanization and external pre-vulcanization technology. The external presulfurization technology can be divided into two types according to the state of the metal on the catalyst: one is that during the external presulfuriz...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J33/00C10G45/04
CPCB01J33/00C10G45/04C10G2300/705C10G2300/202
Inventor 徐黎明高玉兰佟佳杨涛杨占林
Owner CHINA PETROLEUM & CHEM CORP