Fluorescent probe material as well as preparation method and application thereof
A fluorescent probe and solvothermal reaction technology, applied in the field of its preparation and fluorescent probe materials, can solve the problems of high storage requirements, less ability to detect heavy metal ions at the same time, insufficient environmental adaptability, etc., and achieve the effect of high application value.
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[0036] The embodiment of the present invention also proposes a method for preparing a fluorescent probe material, which includes: mixing 1,4-naphthalene dicarboxylic acid, a source of rare earth europium, and N,N-dimethylformamide for solvothermal reaction to obtain the above-mentioned Red-emitting crystalline fluorescent probe material.
[0037] In order to further improve the yield of the product, the inventor further optimized the selection and consumption of raw materials in the preparation method:
[0038] The rare earth europium source is a trivalent europium salt, the rare earth europium source is calculated based on the number of moles of europium ions it contains, and the molar ratio of 1,4-naphthalene dicarboxylic acid to the rare earth europium source is 2:1 to 4, preferably 2:1 ~3. The molar ratio of 1,4-naphthalene dicarboxylic acid and rare earth europium source can be 2:1, 2:2, 2:3, 2:4, etc., or any value between the above adjacent ratio values .
[0039] 1mm...
Embodiment 1
[0049] This embodiment provides a method for preparing a crystalline fluorescent probe material, comprising the following steps:
[0050] Place 4.32g (20mmol) of 1,4-naphthalene dicarboxylic acid and 4.46g (10mmol) of europium nitrate hexahydrate in a 250mL polytetrafluoroethylene liner, then add 150mL of analytically pure N,N-dimethyl Formamide, cover the inner cover, put it into a steel reaction kettle and tighten it, and carry out solvothermal reaction, the reaction temperature is 100 ° C, the reaction time is 2 days, after the reaction is completed, cool to room temperature, filter and wash to obtain a colorless light transparent Bulk crystal Eu(ndc)(Hndc)(DMF) 2 ] n , the yield is greater than 95% (based on the metal salt), named as sample 1#.
Embodiment 2
[0052] This example provides a method for preparing a crystalline fluorescent probe material. The specific steps are roughly the same as those in Example 1, except that the reaction temperature is 90° C., and it is named as sample 2#.
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