Non-linear materials and related devices
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[0052]FIG. 1(a) shows a comparison between ‘Fermi smearing’ and two-photon non-linear responses in gold. The dominant mechanism of gold's cubic non-linearity is the so-called ‘Fermi-smearing’ process in which light absorption at a frequency ωp leads to a non-equilibrium redistribution of electrons near the Fermi level (EF). When probed at ωs this Fermi-smearing has most impact on transitions between the d-band states lying ΔE=2.4 eV below the Fermi level to states above the Fermi level, as illustrated in the left-hand part of FIG. 1(a). Fermi-smearing leads to a very strong cubic optical non-linearity and non-linear absorption (β˜10−5 m / W) peaking at a wavelength of about 516 nm. However this non-linearity is relatively slow as it depends on the thermalization of the hot electron ensemble, which occurs over a period of several picoseconds. To engineer a much faster non-linear medium, we engage the less efficient but ‘instantaneous’ non-linear process of direct non-resonant two-photo...
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