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Method for manufacturing carbon fiber surface titanium dioxide coating

A technology of titanium dioxide and carbon fiber, which is applied in the fields of carbon fiber, fiber treatment, textiles and papermaking, etc., can solve the problems of complex equipment, carbon fiber surface damage, unsuitable for large-scale production, etc., and achieve the effect of smooth and smooth coating

Inactive Publication Date: 2008-08-27
SHANGHAI JIAO TONG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] After searching the literature of the prior art, it was found that Dong Xingguang et al published "High Temperature Oxidation of Carbon Fiber Coated by Radio Frequency Method" in "Fiber Composite Materials" (2005, 03, 28-31 pages), in which it was proposed to use radio frequency method to prepare The anti-oxidation coating on the surface of carbon fiber, the specific method is: heating the carbon fiber by radio frequency at 700-800°C for chemical vapor deposition. mass production

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0022] Example 1: Take 10 g of tetra-IM titanate, 2 g of water, and 60 g of methanol, add acetic acid to make the solution pH=3, and stir for 2 hours to obtain a titanium dioxide precursor solution.

[0023] The carbon fibers are produced by Jilin Carbon Factory, with a diameter of 6-8 μm, and each bundle of carbon fibers has 1000 monofilaments.

[0024] After the carbon fiber bundles were soaked in acetone for 2 minutes, rinsed with deionized water and dried, they were soaked in 10% (volume concentration) nitric acid for 20 minutes for surface oxidation etching, and then infiltrated with the above-mentioned titanium dioxide precursor solution for 5 minutes. Ultrasonic vibration at 120kHz. The cellulose bundle was separated from the precursor at a speed of 0.5mm / s, and the excess precursor on the surface was removed by mechanical extrusion, dried at room temperature for 10 minutes, heated to 100°C at a rate of 4°C per minute, and then held at a constant temperature for 30 minu...

example 2

[0025] Example 2: Carbon fiber is the same as Example 1.

[0026] Take 10 g of tetra-IM titanate, 2 g of water, and 80 g of ethanol, add acetic acid to make the solution pH=3, and stir for 4 hours to obtain a titanium dioxide precursor solution.

[0027] After the carbon fiber bundles were soaked in acetone for 2 minutes, rinsed with deionized water and dried, they were soaked in 10% (volume concentration) nitric acid for 20 minutes for surface oxidation etching, and then infiltrated with the above-mentioned titanium dioxide precursor solution for 15 minutes. The precursor is separated from the precursor at a speed of 10mm / s, and the excess precursor on the surface is removed by drying, dried at room temperature for 20 minutes, heated to 120°C at a rate of 4°C per minute, and kept at a constant temperature for 30 minutes. After the fiber bundle is cooled to room temperature After repeating the above process of infiltration, drying and heating of the precursor once, the tempera...

example 3

[0028] Example 3: Carbon fiber is the same as Example 1.

[0029] Take 10 g of tetra-IM titanate, 2 g of water, and 80 g of n-butanol, add acetic acid to make the solution pH=3, and stir for 4 hours to obtain a titanium dioxide precursor solution.

[0030] The carbon fiber bundles were soaked in acetone for 2 minutes, rinsed with deionized water and dried, and then soaked in 10% (volume concentration) nitric acid for 20 minutes for surface oxidation etching. The excess precursor on the surface was removed by sucking dry, and the above-mentioned titanium dioxide precursor solution was infiltrated for 30 minutes, and the infiltration process was ultrasonically oscillated at 120 kHz. After the cellulose bundle was taken out, it was dried at room temperature for 10 minutes, heated to 150°C at a rate of 4°C per minute, and then kept at a constant temperature for 60 minutes. The temperature was raised to 450°C at a rate of 4°C per minute, then kept at a constant temperature for 60 ...

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Abstract

A method for preparing carbon fiber surface titanium dioxide coating belongs to the material technique field. The invention adopts alcohol as solvent and enables butyl titanate to do hydrolysis reaction to form titanium dioxide forerunner solution. The obtained titanium dioxide forerunner solution is applied and impregnated by predisposed carbon fiber, and then the solvent is evaporated by heating slowly, and a titanium dioxide coating is formed on the carbon fiber filament surface after sintering. The prepared obtained coating thickness is less than 1 mum and the coating is flat and doesn't desquamate easily. On the one hand the carbon fiber of the invention keeps compliance and stitchability of the prior carbon fiber, simultaneously improves thermal oxidation resistance and also improves soakage with a base in the composite material preparation.

Description

technical field [0001] The invention relates to a preparation method in the technical field of composite materials, in particular to a preparation method of a titanium dioxide coating on the surface of carbon fibers. Background technique [0002] Carbon fiber is a commonly used reinforcing fiber for composite materials. It has excellent characteristics such as low density, high strength, high modulus, low thermal expansion, radiation resistance, easy processing, and good thermal and electrical properties. widely used in matrix composites. However, the oxidation resistance of carbon fiber is poor. In the air above 400 ℃, there will be obvious weight loss and strength reduction, and the wettability of carbon fiber and some substrates is not good, so it is difficult to form a dense and excellent composite material. Therefore, it hinders the application of carbon fiber in aerospace and other fields that require lightweight, high-strength, and high-modulus materials. Forming a ...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): D06M11/46D06M101/40
Inventor 夏存娟王浩伟
Owner SHANGHAI JIAO TONG UNIV