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Method for preparing double-pore enzyme immobilization reactor

A technology of enzyme immobilization and reactor, applied to chemical instruments and methods, fixed on/in organic carriers, water/sludge/sewage treatment, etc., to achieve easy recycling, high fluid permeability, overcome The effect of poor loading parallelism

Inactive Publication Date: 2008-09-10
NANKAI UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Since they are usually fine powders with a particle size of 1-15 μm, although they have a large surface area, they also have great defects in practical applications

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0016] Example 1: In a beaker, add 50mL of acetic acid aqueous solution with a pH of 5.0, then add 4.9g of polyethylene glycol, stir, add 24mL of tetramethoxysilane, stir at 0°C for 10min, add 0.1g of hexadecyl Trimethylammonium bromide, continue stirring at 0°C for 30min. The resulting mixture was poured into several polytetrafluoroethylene test tubes, placed in a 40°C water bath, and aged for 24 hours after reaching the gel point to obtain a wet silica gel column. Put the silica gel column after demoulding and rinsing in a constant temperature box, dry at 70°C for 12 hours, strictly control the water loss rate of the colloid, and then bake it in a box-type resistance furnace at 1°C min -1 The temperature was raised to 550° C. at a constant temperature for 4 hours to prepare a monolithic column of double-hole silica gel. The prepared double-hole monolithic column was placed in a polytetrafluoroethylene heat-shrinkable tube, and reacted at 180° C. for 4 hours to complete the ...

Embodiment 2

[0017] Example 2: In a beaker, add 50 mL of acetic acid aqueous solution with a pH of 5.0, then add 4.0 g of polyethylene glycol, stir, add 30 mL of tetramethoxysilane, and stir at 0° C. for 10 min. The resulting mixture was poured into several polytetrafluoroethylene test tubes, placed in a 40°C water bath, and aged for 24 hours after reaching the gel point to obtain a wet silica gel column. Soak the silica gel column after demoulding and rinsing in 0.01mol / L ammonia water, heat treatment at 120°C for 6 hours, then place it in a constant temperature box, and dry it at 70°C for 12 hours to strictly control the dehydration rate of the colloid, and then place it in the box-type resistor Roasting in the furnace at 1°C min -1 The temperature was raised to 550° C. at a constant temperature for 4 hours to prepare a monolithic column of double-hole silica gel. The prepared double-hole monolithic column was placed in a polytetrafluoroethylene heat-shrinkable tube, and reacted at 160°...

Embodiment 3

[0018] Example 3: In a beaker, add 50mL of acetic acid aqueous solution with a pH of 5.0, then add 5.2g of polyethylene glycol, stir, add 36mL of tetraethoxysilane, stir at 0°C for 10min, add 0.29g of citric acid, continue Stir at 0°C for 30 min, and adjust the pH of the solution to 5.0 with ammonia water. The resulting mixture was poured into several polytetrafluoroethylene test tubes, placed in a 40°C water bath, and aged for 24 hours after reaching the gel point to obtain a wet silica gel column. Put the silica gel column after demoulding and rinsing in a constant temperature box, dry at 70°C for 12 hours, strictly control the water loss rate of the colloid, and then bake it in a box-type resistance furnace at 1°C min -1 The temperature was raised to 550° C. at a constant temperature for 4 hours to prepare a monolithic column of double-hole silica gel. The prepared double-hole monolithic column was placed in a polytetrafluoroethylene heat-shrinkable tube, and reacted at 18...

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PUM

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Abstract

The invention provides a preparation method for a diplopore enzyme immobilization reactor, wherein, alkoxy silanes are used as silicon sources; polyethylene glycols are used as macroporous template agents; cetyltrimethylammonium bromides, ammonia or citric acids are used as mesopore template agents; a diplopore silica gel overall carrier is prepared through demoulding, cleaning, drying and baking by adoption of the improved sol-gel method; the silica gel overall carrier is arranged inside a heat contraction tube and closely coated after heating; the silica gel overall carrier after coating is cleaned by utilization of reagents which contain 3-amino propyl triethoxysilane; amido is bonded on the surface of silica gel; the aminated silica gel is cleaned by glutaraldehyde solution and then cleaned by water solution which contains horse-radish catalases, and then the diplopore enzyme immobilization reactor is prepared. The product of the invention can be used for processing waste water which contains persistent organic pollutants and has the advantages of low cost, high efficiency, safe reaction and capability of being reused.

Description

technical field [0001] The invention relates to a preparation method of a dual-hole enzyme immobilization reactor. Background technique [0002] With the rapid development of economy and society, people pay more and more attention to the harm of environmental pollution. The essence of environmental pollution is that a large amount of pollutants are discharged into the environment during human activities, which affects its self-purification ability and disrupts the function of the ecosystem. Among the various chemicals introduced into the environment, persistent organic pollutants are of particular concern. Because of its long-term residue, bioaccumulation, semi-volatility and high toxicity, it has serious harm to the environment and human health. [0003] The degradation technology of persistent organic pollutants has been widely studied at home and abroad, and the commonly used methods are: biological method and chemical method. However, the existing processing technolog...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C12N11/04C02F3/00
Inventor 马小东孙红文王淑荣
Owner NANKAI UNIV