Cationic fluorinated polymer compositions and methods of treating hydrocarbon-bearing formations using same
A technology of fluorinated polymer and composition, which can be used in drilling compositions, chemical instruments and methods, earth-moving drilling, etc., and can solve problems such as unsatisfactory downhole conditions
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[0195] In the following examples, MeFBSEA was prepared according to the method of Parts A and B of Example 2 of U.S. Patent No. 6,664,354 (Savu), except that 4270 kilograms (kg) of N-methylperfluorobutanesulfonamide ethanol, 1.6 kg phenothiazine, 2.7 kg methoxyhydroquinone, 1590 kg heptane, 1030 kg acrylic acid, 89 kg methanesulfonic acid (in place of trifluoromethanesulfonic acid) and 7590 kg water (in part B).
[0196] In the following examples, 3,3,4,4,5,5,6,6,7,7,8,8,8-tridecafluorooctyl acrylate (FOA) was prepared according to the following method. Add 100 g (0.275 mol) of 1H,1H,2H,2H-perfluorooct-1-ol (C 6 f 13 C 2 h 4 OH) (available from Clariant Chemical Co. (Mount Holly, NC) under the trade designation "FLUOWETEA 600"), 19.8 grams (0.275 moles) of acrylic acid (available from Sigma-Aldrich (St. Louis, MO)), 250 grams of heptane, and 1 gram of methane sulfonic acid, and the mixture was heated to reflux for 15 hours. Water (approximately 4.9 to 5 grams) was collect...
example 6 and 7
[0204] The preparation of Examples 6 and 7 was carried out according to the method of Examples 1 to 5, except that 30 grams of solvent mixture was used, the amounts of reagents used and the molar and weight ratios are given in Table 3 below.
[0205] table 3
[0206]
[0207] The gram loss during polymerization and the percent solids of the resulting polymer are given in Table 3 above.
[0208] Examples 8 to 11
[0209] Into each of five 0.1 liter (4 oz) pressure bottles was placed DMAEAMCl (80% by weight in water, available from Ciba Specialty Chemicals under the trade designation "CIBAAGEFLEXFA1Q80MC") and MeFBSEA or FOA in the amounts shown in Table 4 below. For Examples 8 and 9, a mixture of 90 grams of methanol, 90 grams of methyl ethyl ketone, 3 grams of 3-mercapto-1,2-propanediol and 0.60 grams of 2,2'-azobis(2-methylbutyronitrile) was prepared batch. For Examples 10 and 11, a mixture of 45 grams of methanol, 45 grams of methyl ethyl ketone, 1.5 grams of 3-mer...
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