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Preparation method and application of calcium oxide based absorbing material using diatomite as carrier

An absorption material, calcium oxide technology, applied in chemical instruments and methods, through adsorption, other chemical processes, etc., can solve problems that have not yet been seen, and achieve the improvement of cycle absorption stability, reduction of environmental treatment costs, and mitigation of the greenhouse effect. Effect

Inactive Publication Date: 2014-11-05
KUNMING UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

So far, it has not been seen to use the cheap natural mineral diatomaceous earth as a carrier to prepare high-temperature CO 2 Reports on invention patents and research literature of calcium oxide-based absorbent materials

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] Example 1: The preparation method and application of the calcium oxide-based absorbent material using diatomaceous earth as a carrier, the specific content is as follows:

[0024] (1) Roast Yunnan Xianfeng diatomite at 200℃ for 4 hours;

[0025] (2) Put 15ml of Na 2 CO 3 The solution is immersed in 1.5g diatomaceous earth for 2h, and then 15ml CaCl 2 The solution was added to the impregnation mixture, stirred and reacted for 1 hour, filtered with suction, dried at 100°C, and calcined at 750°C for 2 hours to obtain a calcium oxide-based absorbent material with a load of 30%, in which Na 2 CO 3 The concentration of the solution is 0.5mol / L, CaCl 2 The concentration of the solution is 1mol / L.

[0026] (3) Put the prepared calcium oxide-based absorbent material into the thermogravimetric analyzer, and place it in the CO 2 :N 2 =1 (molar ratio) in an atmosphere with a temperature rise rate of 10K / min, the temperature is increased from 40°C to 820°C, and the temperature is kept const...

Embodiment 2

[0027] Embodiment 2: The preparation method and application of the calcium oxide-based absorbent material using diatomaceous earth as a carrier, the specific content is as follows:

[0028] (1) Roast Yunnan Xianfeng Diatomite at 350℃ for 3 h;

[0029] (2) Put 15ml of Na 2 CO 3 The solution is immersed in 1.5g diatomaceous earth for 2h, and then 15ml CaCl 2 The solution was added to the impregnation mixture, stirred and reacted for 1 hour, filtered with suction, dried at 100°C, and calcined at 700°C for 4 hours to obtain a calcium oxide-based absorbent material with a loading capacity of 30%. 2 CO 3 The concentration of the solution is 1.5mol / L, CaCl 2 The concentration of the solution is 2mol / L.

[0030] (3) Put the prepared calcium oxide-based absorbent material into the thermogravimetric analyzer, and place it in the CO 2 :N 2 =1 (molar ratio) in an atmosphere with a temperature rise rate of 10K / min, the temperature is increased from 40°C to 820°C, and the temperature is kept consta...

Embodiment 3

[0031] Embodiment 3: The preparation method and application of the calcium oxide-based absorbent material using diatomaceous earth as a carrier, the specific content is as follows:

[0032] (1) Roast Yunnan Xianfeng diatomite at 500℃ for 2 h;

[0033] (2) Put 12ml of Na 2 CO 3 The solution is immersed in 1.5g diatomaceous earth for 4h, then 24ml CaCl 2 The solution was added to the impregnation mixture, stirred for 2h, filtered with suction, dried at 100°C, and calcined at 650°C for 8h to obtain a calcium oxide-based absorbent material with a loading capacity of 30%. 2 CO 3 The concentration of the solution is 2.5mol / L, CaCl 2 The concentration of the solution is 0.5mol / L.

[0034] (3) Put the prepared calcium oxide-based absorbent material into the thermogravimetric analyzer, and place it in the CO 2 :N 2 =5 (molar ratio) in an atmosphere, raise the temperature from 40°C to 700°C at a heating rate of 10K / min, and keep it constant for 45min to perform CO 2 Absorption reaction, the res...

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Abstract

The invention discloses a preparation method of calcium oxide based absorbing materials using diatomite as carriers. The preparation method uses natural minerals diatomite as the carriers and supported calcium oxide based materials are synthesized through impregnation and precipitation methods. Under high-temperature conditions, the calcium oxide based materials prepared by adopting the method can absorb CO2 in mixed gas of CO2 and N2. Compared with the prior art, the carrier material, i.e. the diatomite used in the method is cheap and is easy to obtain, the prepared adsorbents have the advantages of high CO2 absorbing capacity and high adsorbing stability in the multi-time circulation process, the greenhouse effect is relieved, the CO2 emission is reduced and the environmental improvement cost is reduced.

Description

Technical field [0001] The invention relates to a preparation method and application of a calcium oxide-based absorption material using diatomaceous earth as a carrier, and belongs to the absorption and separation of high-temperature CO discharged from power plants and flue gas 2 field. Background technique [0002] In recent years, with the rapid economic development of various countries, CO 2 The emissions of CO 2 The greenhouse gas effect caused has attracted widespread attention all over the world. CO emissions from fossil fuel power plants 2 The amount of CO caused by various human activities 2 More than 30% of total emissions are CO 2 The largest fixed source of emissions, so the CO emissions from thermal power plants are controlled and recovered 2 It is of great significance to solve the problem of greenhouse effect. Due to the higher temperature of the gas discharged from high-temperature furnaces such as thermal power plants, the CO in the flue gas 2 The separation of ca...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/32B01J20/14
CPCY02C10/08Y02C20/40
Inventor 陕绍云贾庆明蒋丽红王亚明彭金辉
Owner KUNMING UNIV OF SCI & TECH