Method for preparing spongy porous silicon material
A porous silicon and sponge-like technology, applied in chemical instruments and methods, silicon compounds, inorganic chemistry, etc., can solve problems such as the production method of sponge-like porous silicon materials that have not yet appeared, and achieve regular pore shape, improved performance, and uniform layout Effect
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Embodiment 1
[0035] Purification of diatomite: Diatomite (silicon dioxide content between 80-90%) is soaked in sulfuric acid, nitric acid or hydrochloric acid for 5-10 hours to remove water-soluble impurities, and then mixed with ammonium sulfate at a ratio of 95-98% to 5 %-2% by weight and mixed evenly, at 400 ℃ - 600 ℃, calcined in air for 2 hours - 4 hours, after cooling, stir and filter with deionized water to remove water-soluble impurities, at 80 ℃ - 120 ℃ Dry to obtain purified diatomaceous earth.
[0036] Diatomite reduction: the purified diatomite and sodium, potassium, magnesium or calcium are directly reduced at a ratio of 25% or higher than the chemical equivalent in a protective gas of argon at 600°C-800°C at high temperature4 Hours to 6 hours, the reaction product is neutralized with hydrochloric acid aqueous solution, leached to remove sodium, potassium, magnesium or calcium chloride, filtered, washed with water, and dried at 80°C-120°C to obtain a high-purity sponge porous...
Embodiment 2
[0041] Purification of diatomite: Soak 600 grams of diatomite (silicon dioxide content between 80-90%) and 12000 grams with sulfuric acid, nitric acid or hydrochloric acid for 5-10 hours to remove water-soluble impurities, and then mix with 60 grams of sulfuric acid After the ammonium is mixed evenly, it is calcined in the air at 400 ℃ - 600 ℃ for 2 hours - 4 hours, after cooling, it is stirred with deionized water and filtered to remove water-soluble impurities, and dried at 80 ℃ - 120 ℃ to obtain purified diatoms earth.
[0042] Diatomaceous earth reduction: the purified diatomite and 900 grams of calcium are directly reduced in the protective gas of argon at 600 ° C to 800 ° C for 4 hours to 6 hours, and the reaction product is neutralized with hydrochloric acid aqueous solution, soaked Remove sodium, potassium, magnesium or calcium chloride, filter, wash with water, and dry at 80°C-120°C to obtain high-purity sponge-like porous silicon.
[0043] Taking calcium as a reduci...
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