Curable resin composition, its sheet, molded body, semiconductor package, semiconductor component, and light-emitting diode
A technology of light-emitting diodes and curable resins, applied in semiconductor/solid-state device parts, semiconductor devices, electric solid-state devices, etc., can solve the problems of reduced fluidity, reduced resin strength, and damage to molding processability, etc., to achieve low linear expansion coefficient, reduced warpage, and excellent toughness
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[0411] Hereinafter, examples and comparative examples of the present invention are shown, but the present invention is not limited by the following contents.
Synthetic example 1
[0413] 200 g of toluene and 50 g of 1,3,5,7-tetramethylcyclotetrasiloxane were placed in a 500 mL four-necked flask, and the gas phase was replaced with nitrogen, followed by heating and stirring at an internal temperature of 105°C. Add 11.0 g of diallyl monoglycidyl isocyanurate, 11.0 g of toluene, and 0.0162 g of a xylene solution (containing 3% by weight as platinum) of vinylsiloxane-platinum complex dropwise over 30 minutes. Mixture. After 6 hours from the end of the dropwise addition, by 1 H-NMR confirmed that the reaction rate of the allyl group was 95% or more, and the reaction was terminated by cooling. Unreacted 1,3,5,7-tetramethylcyclotetrasiloxane and toluene were distilled off under reduced pressure to obtain a colorless and transparent liquid. pass 1 H-NMR measurement shows that this liquid is a part of SiH group of 1,3,5,7-tetramethylcyclotetrasiloxane reacted with diallyl monoglycidyl isocyanurate and has the following properties: structured matter. In addi...
Synthetic example 2
[0417] A stirring device, a dropping funnel, and a condenser were installed in a 5 L four-necked flask. 1,800 g of toluene and 1,440 g of 1,3,5,7-tetramethylcyclotetrasiloxane were placed in the flask, and heated and stirred in a 120° C. oil bath. A mixed solution of 200 g of triallyl isocyanurate, 200 g of toluene, and 1.44 ml of a xylene solution (containing 3% by weight as platinum) of a vinylsiloxane-platinum complex was added dropwise over 50 minutes. After heating and stirring the obtained solution for 6 hours as it was, unreacted 1,3,5,7-tetramethylcyclotetrasiloxane and toluene were distilled off under reduced pressure. pass 1 H-NMR measurement revealed that this liquid had the following structure obtained by reacting some SiH groups of 1,3,5,7-tetramethylcyclotetrasiloxane and triallyl isocyanurate.
[0418] [chemical formula 20]
[0419]
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