Magneto-optical double-mode imaging nanoprobe and application thereof
A magneto-optical dual-mode, nano-probe technology, applied in the field of biomedicine, can solve the problem of not being able to provide information on the structure and function of biological tissues, achieve good blood circulation time in the body, good clinical transformation prospects, and easy surface functional modification Effect
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Embodiment 1
[0031] NIR Ag 2 S quantum dots: The surface ligand is lipoic acid, with an average of about 5.4nm. The preparation method is as follows: 0.1 mmol of silver diethyldithiocarbamate and 10 g of dodecanethiol are mixed and placed in a flask, and placed in a flask under N 2 The temperature was raised to 200°C in the atmosphere and kept for 1 hour. Finally, after the solution was naturally cooled to room temperature, 50 mL of absolute ethanol was added, centrifuged, washed, dispersed in cyclohexane, and then an equal volume of absolute ethanol was added to the solution in an ultrasonic cleaner. Sonicate for 4h, then centrifuge, and wash with deionized water to obtain water-soluble Ag with a particle size of about 5nm 2 S quantum dots.
[0032] Preparation of a magneto-optical dual-mode nanoprobe: a near-infrared Ag 2 S quantum dots, Gd-DOTA, are assembled by amino-functionalized PEG molecules. Among them, Gd-DOTA was purchased from Sigma, and amino-functionalized modified PEG wa...
Embodiment 2
[0044] NIR Ag 2 Se quantum dots: the surface ligand is C18-PMH-PEG, with an average size of 3.5nm. The preparation method is as follows: add 0.04mmol Ag-Oleylamine, 7mL toluene, 3mL dodecanethiol, and 7mL 0.01mmol / L NaHSe solution into a 50mL reactor and stir for 5min, then place it at 180°C for 1h. Then use 60mL absolute ethanol, centrifuge, wash, disperse in chloroform, then add 50mgDSPE-PEG-NH 2 (purchased from Nanocs) and stirred for 12h, finally washed by centrifugation and dispersed in water.
[0045] Fabrication of magneto-optical dual-mode nanoprobes: from near-infrared Ag 2 Se quantum dots and Gd-DTAP were assembled by amino-functionalized PEG molecules. Among them, Gd-DTPA was purchased from Sigma, and amino-functionalized modified PEG was purchased from Sunbio.
[0046] Its preparation method is as follows.
[0047] (1) Chemically cross-linked Gd chelate molecules and modified PEG molecules: 50mgGd-DTAP, 100mgDSPE-PEG-NH 2 , add 10 mL containing 75 mM EDC (1-e...
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