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Method of toughening polypropylene with compound nucleating agent

The technology of polypropylene and nucleating agent is applied in the field of compound nucleating agent to toughen polypropylene, which can solve the problems of high addition cost, increase the cost of composite materials, reduce the rigidity and transparency of polypropylene, etc., so as to reduce the dosage and improve the toughness. , The effect of toughening effect is obvious

Inactive Publication Date: 2018-04-13
SHAANXI RES DESIGN INST OF PETROLEUM CHEM IND
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The formation of β-crystal polypropylene mainly includes three methods: temperature method, shear orientation method and adding nucleating agent. Among them, adding β-crystal nucleating agent to polypropylene has become a method to obtain polypropylene with high β-crystal content. A practical and effective method, but the cost of single addition is relatively high
[0004] In recent years, the use of elastomers to modify and toughen polypropylene has become a common method, but only when the amount of elastomer added is greater than 20 parts, the toughening effect can be clearly shown. The cost of the material and at the expense of reducing the rigidity and transparency of polypropylene while toughening

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] 1) Adding mass parts in the reactor is 78 parts by mass of polybutadiene latex, 10 parts by mass of methyl methacrylate monomer, 4 parts by mass of sodium pyrophosphate, 3 parts by mass of glucose and 3 ferrous sulfate, under the action of cumene hydroperoxide as an initiator in the number of parts by mass, the above-mentioned substances were grafted and polymerized at 70°C for 6 hours to obtain PB-g-PMMA latex;

[0028] 2) Pour the latex into 15% sulfuric acid solution, adjust the pH to about 5, raise the temperature to 70°C, stir for 30min, and cool to room temperature. High-speed centrifugation to remove water, wash with distilled water, and dry at 50°C for 24 hours to obtain powdered nano-core-shell PB-g-PMMA particles with a particle size of 60-200nm;

[0029] 3) 55.99 parts of random copolymerized polypropylene, 35 parts of syndiotactic homopolymerized polypropylene, 5 parts of nano core-shell PB-g-PMMA particles, 0.01 part of TMB-4 nucleating agent (developed by ...

Embodiment 2

[0032] 1) Adding mass parts in the reactor is 65 parts by mass of polybutadiene latex, 15 parts by mass of methyl methacrylate monomer, 5 parts by mass of sodium pyrophosphate, 7 parts by mass of glucose and 7 ferrous sulfate, under the action of cumene hydroperoxide as an initiator in the number of parts by mass, the above substances were grafted and polymerized at 70°C for 8 hours to obtain PB-g-PMMA latex;

[0033] 2) Pour the latex into 20% sulfuric acid solution, adjust the pH to about 2, raise the temperature to 70°C, stir for 30min, and cool to room temperature. High-speed centrifugation to remove water, wash with distilled water, and dry at 50°C for 24 hours to obtain powdered nano-core-shell PB-g-PMMA particles;

[0034] 3) 70 parts of random copolymerized polypropylene, 20 parts of block copolymerized polypropylene, 4 parts of nano core-shell PB-g-PMMA particles, 0.04 parts of WBG-II nucleating agent (Guangdong Weilinna New Material Technology Co., Ltd. Production, ...

Embodiment 3

[0037] 1) Adding mass parts in the reactor is 80 parts by mass of polybutadiene latex, 5 parts by mass of methyl methacrylate monomer, 5 parts by mass of sodium pyrophosphate, 4 parts by mass of glucose and 4 ferrous sulfate, under the action of cumene hydroperoxide as an initiator in the number of parts by mass, the above-mentioned substances were grafted and polymerized at 70°C for 10 hours to obtain PB-g-PMMA latex;

[0038] 2) Pour the latex into 15% sulfuric acid solution, adjust the pH to about 5, raise the temperature to 70°C, stir for 30min, and cool to room temperature. High-speed centrifugation to remove water, wash with distilled water, and dry at 50°C for 24 hours to obtain powdered nano-core-shell PB-g-PMMA particles;

[0039]3) 60 parts of block copolymerized polypropylene, 30.98 parts of syndiotactic homopolymerized polypropylene, 5 parts of nano core-shell PB-g-PMMA particles, 0.02 parts of TMB-5 nucleating agent (developed by Shanxi Chemical Industry Research ...

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Abstract

The invention relates to a method for toughening polypropylene with a compound nucleating agent. The method comprises the following steps: mixing the following components at a high speed: 75 to 95 parts of polypropylene resin, 1 to 10 parts of nanometer core-shell particles, 0 to 0.5 part of a beta nulceaing agent, 1 to 10 parts of a surface modifier, 1 to 5 parts of an antioxidant and 0 to 3 parts of a dispersant, and carrying out mixing, extrusion and granulation so as to obtain toughened polypropylene particles. According to the invention, through addition of the nanometer core-shell particles and the beta nucleating agent for coordinative toughening of a polypropylene material, the effect of toughening is significant; rigidity and toughness are well balanced; the cost is reduced; and efficiency is improved. The polypropylene material prepared by using the method provided by the invention has excellent impact toughness, good rigidity, high thermal deformation temperature, and insusceptibility to brittle fracture at a low temperature. Performance test results show that the toughened polypropylene prepared by using the method provided by the invention has notched impact strength of 58.1 KJ / m2, elongation at break of 790% and flexural modulus of 1520 MPa. The toughened polypropylene prepared by using the method provided by the invention has wide application range and is appliedto the fields of daily necessities, automobiles, household appliances, medical apparatus and instruments, etc.

Description

technical field [0001] The invention relates to a method for compounding a nucleating agent to toughen polypropylene. Background technique [0002] Polypropylene is a widely used thermoplastic resin. It combines excellent mechanical properties and low cost. It has strong non-toxic and chemical corrosion resistance. It has broad market prospects and has become the fastest growing among the five general-purpose synthetic resins. , the most active species. However, due to its typical non-polarity and high crystallinity, polypropylene products are unsatisfactory in terms of impact toughness, low heat distortion temperature, and easy to be brittle at low temperature. The industrial application of high added value of polypropylene is limited. [0003] Polypropylene has a variety of crystal forms, namely α, β, γ, δ and pseudo-hexagonal crystal. Among them, the α crystal form is the most common, and other crystal forms can only be obtained under special circumstances, such as she...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08L23/14C08L23/12C08L53/00C08L51/04C08L23/06C08K5/18C08K5/544C08K5/134C08K5/00C08F279/02
CPCC08F279/02C08L23/14C08L53/00C08L2205/03C08L2205/035C08L23/12C08L51/04C08L23/06C08K5/18C08K5/544C08K5/1345C08K5/00
Inventor 王悦黄捷高超锋王波汤粤豫田小艳杨金明
Owner SHAANXI RES DESIGN INST OF PETROLEUM CHEM IND