P-type impurity diffusion composition, method of manufacturing semiconductor element using same, and method of manufacturing solar cell
A technology of impurity diffusion and composition, which is applied in semiconductor/solid-state device manufacturing, semiconductor devices, electrical components, etc., can solve the problems that the gas diffusion method cannot be applied, and achieve excellent barrier properties
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Embodiment 1
[0212] (1) Synthesis of polysiloxane solution
[0213] 164.93 g (1.21 mol) of KBM-13 (manufactured by Shin-Etsu Chemical Co., Ltd., MeTMS), 204.07 g (1.21 mol) of KBM-103 (manufactured by Shin-Etsu Chemical Co., Ltd., PhTMS), and 363.03 g were added to a 1000 mL three-necked bottle. γ-BL was added over 30 minutes, while stirring at 40° C., an aqueous formic acid solution in which 0.1.215 g of formic acid was dissolved in 130.76 g of water. After completion of the dropwise addition, the mixture was stirred at 40° C. for 1 hour, then heated up to 70° C., and stirred for 30 minutes. Thereafter, the temperature of the oil bath was raised to 115°C. One hour after the start of temperature rise, the internal temperature of the solution reached 100° C., and it was heated and stirred for 1 hour thereafter (internal temperature: 100° C. to 110° C.). The resulting solution was cooled in an ice bath to obtain a polysiloxane solution A (PhTMS (50 mol%) / MeTMS (50 mol%), ie a substance hav...
Embodiment 2
[0220] The composition of the polysiloxane is such that n:m=90:10 in the general formula (1), and the feed ratio of the raw materials is PhTMS (90 mol%) / MeTMS (10 mol%). In the same manner as in Example 1, impurity-diffusing composition B was obtained. Using the obtained impurity-diffusing composition B, the peelability, sheet resistance, diffusion uniformity, and barrier properties were measured, and as shown in Table 2, all showed good results. In addition, the weight average molecular weight (Mw) of the polysiloxane in the polysiloxane solution used was 2300.
Embodiment 3
[0222] The composition of the polysiloxane is n:m=80:20 in the general formula (1), and the feed ratio of the raw materials is PhTMS (80 mol%) / MeTMS (20 mol%). In the same manner as Example 1, impurity-diffusing composition C was obtained. Using the obtained impurity-diffusing composition C, the peelability, sheet resistance, diffusion uniformity, and barrier properties were measured, and as shown in Table 2, all showed good results. In addition, the weight average molecular weight (Mw) of the polysiloxane in the polysiloxane solution used was 2500.
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