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Preparation method of high-performance grafted starch

A high-performance, starch technology, applied in the polymer field, to achieve the effect of improving the performance and application range

Active Publication Date: 2019-01-01
JIANGNAN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This enzymatic modification of starch materials based on the idea of ​​"modification of substrate molecular structure" overcomes the "inapplicability" of existing enzyme preparations for starch grafting, and effectively solves the inherent advantage of enzymes in terms of specificity of action technically. cause negative impact

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0042]Add 100mL of acetone to 100mL of phosphate buffer (0.1mol / L, pH=7.5), mix the solution and separate layers, take the acetone containing phosphate in the upper layer and add 50g of diatomaceous earth. min in a shaker for 1 h, filtered and dried at 100°C for 8 h to obtain immobilized phosphate.

[0043] Add 10g of absolute dry cornstarch, 20g of ethylene glycol diacrylate and 30g of the catalyst prepared above into 500mL of dimethyl sulfoxide, react in a constant temperature shaker at 50°C and 200r / min for 24h, add ethanol to precipitate and obtain Vinyl-containing starch monoester products. Dissolve 10g of acrylamide monomer in 500mL of water, add 10g of vinyl-containing corn starch monoester product, then add 1mL of acetylacetone, 0.1mL of H 2 o 2 And 100U of HRP, after reacting for 12h, add ethanol to precipitate to obtain the product of starch grafted acrylamide. The grafting rate was 51.1%.

Embodiment 2

[0045] Add 100mL of acetone to 100mL of phosphate buffer (0.1mol / L, pH=7.5), mix the solution and separate layers, take the acetone containing phosphate in the upper layer and add 50g of diatomaceous earth. min in a shaker for 1 h, filtered and dried at 100°C for 8 h to obtain immobilized phosphate.

[0046] Add 5g of absolute dry potato starch, 15g of ethylene glycol diacrylate and 20g of the catalyst prepared above into 500mL of dimethyl sulfoxide, react in a constant temperature shaker at 50°C and 200r / min for 12h, add ethanol to precipitate and obtain Vinyl-containing starch monoester products. Dissolve 10g of acrylamide monomer in 500mL of water, add 10g of vinyl-containing potato starch monoester product, then add 1mL of acetylacetone, 0.1mL of H 2 o 2 And 200U of HRP, after reacting for 12h, add ethanol to precipitate to obtain the product of starch grafted acrylamide. The grafting rate was 54.6%.

Embodiment 3

[0048] Add 100mL of acetone to 100mL of phosphate buffer (0.1mol / L, pH=7.5), mix the solution and separate layers, take the acetone containing phosphate in the upper layer and add 50g of diatomaceous earth. min in a shaker for 1 h, filtered and dried at 100°C for 8 h to obtain immobilized phosphate.

[0049] Add 5g of absolute-dried tapioca starch, 15g of ethylene glycol diacrylate and 20g of the catalyst prepared above into 500mL of dimethyl sulfoxide, react in a constant temperature shaker at 50°C and 200r / min for 24h, add ethanol to precipitate and obtain Vinyl-containing starch monoester products. Dissolve 10g of acrylamide monomer in 500mL of water, add 10g of vinyl-containing tapioca monoester product, then add 2mL of acetylacetone, 0.2mL of H 2 o 2 And 300U of HRP, after reacting for 6h, add ethanol to precipitate to obtain the product of starch grafted acrylamide. The grafting rate was 59.3%.

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PUM

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Abstract

The invention discloses a preparation method of high-performance grafted starch, and belongs to the technical field of macromolecules. According to the preparation method, firstly, a vinyl anchor point is introduced onto a molecular chain of starch by utilizing a transesterification reaction; afterwards, the high-efficiency starch grafting is catalyzed and initiated by utilizing peroxidase (HRP (Horse Radish Peroxidase)); a vinyl starch modified material with a high grafting ratio is prepared; and the service performance and the application range of enzymatic method grafted starch are improvedand enlarged. By using the preparation method, the problems that the starch lacks a synthetase catalyzed specific group and greatly limits the action effect of an enzyme are solved.

Description

technical field [0001] The invention relates to a method for preparing high-performance grafted starch, which belongs to the technical field of macromolecules. Background technique [0002] Textile starch materials are mainly used as textile auxiliaries (such as adhesives, sizing materials, pastes, finishing agents, etc.). On the one hand, starch materials for textiles have good environmental protection properties, but at the same time, they have great deficiencies or deficiencies in performance and special functions. Therefore, various chemical, physical and biological methods have been used to modify such materials. Among them, biological modification has become the most promising method in the field of material modification due to its unique advantages of specificity, high selectivity and environmental friendliness. [0003] The biological modification of materials has mainly gone through two stages of development: one is the initial stage of hydrolytic modification of s...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08F251/00C08F220/56C08F220/14C08F220/18
CPCC08F251/00C08F220/1804
Inventor 徐进张静雅范雪荣高卫东王强
Owner JIANGNAN UNIV