Spinnable azobenzene polymer energy storage material and preparation method thereof
A technology of energy storage materials and polymers, which is applied in the direction of single-component synthetic polymer rayon, textiles and papermaking, and fiber chemical characteristics, which can solve the problems of low polymer molecular weight and poor film-forming properties of polymers.
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[0018] The present invention designs the preparation method of above-mentioned azobenzene polymer, and described method reaction formula is illustrated as follows:
[0019]
Embodiment 1
[0021] 1) Dissolve 3g of 3,5-dicarboxylic acid aniline and 1.52g of sodium nitrite in deionized water, add 48ml of 1mol / l hydrochloric acid under ice bath conditions, carry out diazotization for half an hour, then add to 2.5g of 3,5- In the dimethoxyphenol solution, keep the pH between 5-7, and react for 8 hours. After the reaction is over, adjust the pH to about 3, filter with suction to obtain the crude product of the filter cake, and use the obtained crude product with deionized water and anhydrous After washing with water and ethanol for several times, 5 μm silica gel was used as the stationary phase, and ethyl acetate / n-hexane was used as the eluent for chromatographic separation. The obtained fraction was distilled under reduced pressure and dried under vacuum to obtain AZO 3g.
[0022] 2) Dissolve 2g of cis-5-norbornene-exo-2,3-dicarboxylic anhydride and 1.6g of 6-aminocaproic acid in 20ml of toluene solution, add 0.1ml of triethylamine dropwise, and heat up to React a...
Embodiment 2
[0025] 1) Dissolve 3g of 3,5-dicarboxylic acid aniline and 1.52g of sodium nitrite in deionized water, add 48ml of 1mol / l hydrochloric acid under ice bath conditions, carry out diazotization for half an hour, then add to 2.5g of 3,5- In the dimethoxyphenol solution, keep the pH between 5-7, and react for 8 hours. After the reaction is over, adjust the pH to about 3, filter with suction to obtain the crude product of the filter cake, and use the obtained crude product with deionized water and anhydrous After washing with water and ethanol for several times, 5 μm silica gel was used as the stationary phase, and ethyl acetate / n-hexane was used as the eluent for chromatographic separation. The obtained fraction was distilled under reduced pressure and dried under vacuum to obtain 2.8 g of AZO.
[0026] 2) Dissolve 2g of cis-5-norbornene-exo-2,3-dicarboxylic anhydride and 1.6g of 6-aminocaproic acid in 20ml of toluene solution, add 0.1ml of triethylamine dropwise, and heat up to R...
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