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Preparation method of Nd and Er co-doped CaBi8Ti7O27 ceramic and product of Nd and Er co-doped CaBi8Ti7O27 ceramic

A cabi8-x-yndxeryti7o27, co-doping technology, applied in the field of bismuth layered ceramics, can solve the problems of large dielectric loss at high temperature, not widely used, poor piezoelectric activity, etc., to improve the compactness and promote the piezoelectric performance. and ferroelectric properties, the effect of a simple preparation method

Active Publication Date: 2020-11-06
宁波晶昭科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] Currently, CaBi 8 Ti 7 o 27 Intergrowth bismuth layered ceramics have attracted extensive attention from researchers because of their unique superlattice structure and high Curie temperature. However, CaBi 8 Ti 7 o 27 The disadvantages of ceramics, such as poor piezoelectric activity and large high-temperature dielectric loss, have not been widely used to a certain extent.

Method used

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Examples

Experimental program
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Effect test

preparation example Construction

[0027] A kind of Nd and Er co-doped CaBi of the present invention 8 Ti 7 o 27 The preparation method of pottery, described preparation method comprises the steps:

[0028] 1) CaCO with a purity greater than 99.0% 3 、 Bi 2 o 3 、TiO 2 、Nd 2 o 3 and Er 2 o 3 Dry at 80-100°C for 20-30 hours respectively;

[0029] 2) The raw material after step 1) is dried according to CaBi 8-x-y Nd x Er y Ti 7 o 27, where x=0.005~0.04, y=0.005~0.04 stoichiometric ratio is weighed, then put in the polyethylene ball mill jar and carry out ball milling with zirconia zirconium ball, described ball milling speed is 300~400r / min, ball milling The time is 20 to 30 hours, wherein the ball milling medium is absolute ethanol;

[0030] 3) After ball milling, dry the obtained mixed material in a vacuum oven at 65-85°C for 10-20 hours to remove ethanol, grind after drying, and pass the ground powder through an 80-mesh sieve;

[0031] 4) Calcinate the sieved powder in a muffle furnace at 800-90...

Embodiment 1

[0034] A kind of Nd and Er co-doped CaBi 8 Ti 7 o 27 The preparation method of pottery, described preparation method comprises the steps:

[0035] 1) CaCO with a purity greater than 99.0% 3 、 Bi 2 o 3 、TiO 2 、Nd 2 o 3 and Er 2 o 3 Dry at 90°C for 25 hours respectively;

[0036] 2) The raw material after step 1) is dried according to CaBi 7.98 Nd 0.01 Er 0.01 Ti 7 o 27 The stoichiometric ratio is weighed, and then placed in a polyethylene ball mill jar for ball milling with zirconium dioxide zirconium balls, the ball milling speed is 350r / min, and the ball milling time is 25h, wherein the ball milling medium is absolute ethanol;

[0037] 3) After the ball milling, dry the obtained mixed material in a vacuum oven at 80° C. for 18 hours to remove ethanol, grind after drying, and pass the ground powder through an 80-mesh sieve;

[0038] 4) The sieved powder was calcined in a muffle furnace at 850°C for 5h, the heating rate was 5°C, cooled to room temperature, and 5...

Embodiment 2

[0040] A kind of Nd and Er co-doped CaBi 8 Ti 7 o 27 The preparation method of pottery, described preparation method comprises the steps:

[0041] 1) CaCO with a purity greater than 99.0% 3 、 Bi 2 o 3 、TiO 2 、Nd 2 o 3 and Er 2 o 3 Dry at 80°C for 30 hours respectively;

[0042] 2) The raw material after step 1) is dried according to CaBi 7.96 Nd 0.02 Er 0.02 Ti 7 o 27 The stoichiometric ratio is weighed, and then placed in a polyethylene ball mill jar for ball milling with zirconium dioxide zirconium balls, the ball milling speed is 400r / min, and the ball milling time is 20h, wherein the ball milling medium is absolute ethanol;

[0043] 3) After ball milling, dry the obtained mixed material in a vacuum oven at 70° C. for 18 hours to remove ethanol, grind after drying, and pass the ground powder through an 80-mesh sieve;

[0044] 4) The sieved powder was calcined in a muffle furnace at 800°C for 6h, the heating rate was 4°C, cooled to room temperature, and 5% po...

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PUM

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Abstract

The invention discloses a preparation method of Nd and Er co-doped CaBi8Ti7O27 ceramic and a product of the Nd and Er co-doped CaBi8Ti7O27 ceramic. The chemical composition of the material is CaBi <8-x-y> Nd <x> Er <y> Ti <7> O <27>, wherein x is equal to 0.005-0.04, and y is equal to 0.005-0.04. Raw materials are weighed according to the above stoichiometric ratios, and ball milling, pre-calcining, secondary ball milling, compression molding, adhesive discharging and sintering are performed to obtain the product. The preparation method is simple; and the piezoelectric property and the ferroelectric property of the product can be effectively improved by doping the CaBi8Ti7O27 ceramic, and the CaBi8Ti7O27 ceramic is an ideal material used in the field of photoelectric multifunctional materials.

Description

technical field [0001] The invention belongs to bismuth layered ceramics, in particular to a kind of Nd and Er co-doped CaBi 8 Ti 7 o 27 Preparation methods and products of ceramics. Background technique [0002] Bi layered ferroelectric materials have high Curie temperature and good anti-fatigue properties, and have high application prospects in the fields of ferroelectric storage and high-temperature piezoelectric devices. The bismuth layered structure ferroelectric material is composed of bismuth poplar layers and perovskite-like layers alternately arranged along the c-axis direction. Due to the particularity of the bismuth oxygen-like structure, the spontaneous polarization is easily restricted by the two-dimensional ab plane, resulting in bismuth layered The coercive field of structural ceramics is high, and the piezoelectric activity is low. In addition, Bi ions will volatilize at high temperatures, resulting in oxygen vacancies, which deteriorate the electrical pro...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C04B35/475C04B35/622C04B35/638
CPCC04B35/475C04B35/622C04B35/638C04B2235/3208C04B2235/3251C04B2235/3224C04B2235/602C04B2235/6562C04B2235/6567
Inventor 邹振卫
Owner 宁波晶昭科技有限公司