Aqueous battery pole piece material, aqueous battery pole piece and preparation method and application of aqueous battery pole piece
A battery pole piece, water system technology, applied in electrode manufacturing, battery electrode, electrode rolling/calendering, etc., can solve the problem of small active material loading, insufficient control of pole piece surface density and compaction density, weight gap, etc. question
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Embodiment I
[0101] Embodiment 1 prepares polyimide active material 1
[0102]Using N-methylpyrrolidone as a solvent, add 1,4,5,8-naphthalene tetracarboxylic anhydride and anhydrous ethylenediamine to the solvent at a molar ratio of 1:1.02 for reaction; the reaction vessel is a glass flask, Under the protection of argon, the reactant was kept at 150° C. for 5 hours, and the product was collected and vacuum-dried at 120° C. to obtain a dry powder, which was designated as polyimide active material I.
Embodiment II
[0103] Embodiment II prepares polyimide active material II
[0104] Add the reactants 1,4,5,8-naphthalene tetracarboxylic dianhydride and ethylenediamine into the reactor at a molar ratio of 1:1, and the reaction vessel is a glass flask. The reactant was kept at 90° C. for 2 hours under the protection of argon, then raised to 150° C., and reacted at this temperature for 4 hours. The resultant was collected and kept at 200° C. under vacuum for 24 hours to obtain a dry powder, which was designated as polyimide active material II.
Embodiment III
[0105] Embodiment III prepares polyimide active material III
[0106] Add tetraformic acid dianhydride powder and ethylenediamine solution into the N-dimethylformamide (DMF) solution at a molar ratio of 1:1, and keep magnetic stirring. The reaction vessel is a glass flask. The flask was protected with argon. The flask was transferred to a 50°C oil bath, and the temperature was gradually raised to 150°C. The reaction is maintained at this temperature for 4 to 18 hours. The resultant was collected, centrifuged, and the supernatant was removed. For the centrifuged sediment below, it was diluted and washed with N-dimethylformamide, and a second centrifugation was performed. Wash and centrifuge twice with ethanol. The final material was dried in a vacuum oven to obtain a dry powder, which was designated as polyimide active material III.
[0107] Infrared spectroscopy is used to test polyimide active materials Ⅰ~III. Typical test results are polyimide active materials I, from ...
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