Yellow fluorescent powder as well as preparation method and use method thereof
A technology of yellow phosphor powder and light-emitting device, applied in the field of yellow phosphor powder and its preparation, can solve the problems of low luminous efficiency of nano-phosphor powder, complicated process of nano-phosphor powder and high cost, and achieves reduction of synthesis cost and environmental pollution, The effect of superior luminous performance
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[0029] The methods used in the prior art for the preparation of phosphors include: high-temperature solid-state reaction method, co-precipitation method to prepare precursors, sol-gel method and combustion method.
[0030] The high-temperature solid-state reaction method is a reaction method in which solid particles are mixed and sintered at a temperature below the melting point. In the solid state sintering process of the unit system, except for the bonding between powder particles, densification and the change of the structure of pure metal, there is no dissolution between the structures, and there is no new composition or new phase. Within the range of temperature control, the high-temperature solid-phase reaction method is stable, easy to operate and less required for the reaction. However, during the implementation of the high-temperature solid-state reaction method, if the particle size of the participating substances is large, there will be a phenomenon of component seg...
Embodiment 1
[0047] A kind of yellow fluorescent powder, its chemical formula is: Bi 1-x Ca 3 (PO 4 ) 3 O:xDy 3+ , where x=0.01. The above yellow phosphor Bi 0.99 Ca 3 (PO 4 ) 3 O:0.01Dy 3+ The preparation method:
[0048] Weigh CaCO 3 : 3g, Bi 2 o 3 : 230.67g, NH 4 h 2 PO 4 : 3.451g, Dy 2 o 3 : 1.865g. Put the above compound into a quartz mortar and crush it by means of grinding and mixing evenly, then transfer it to a crucible or other heating reaction device and place it in a muffle furnace, and pre-sinter it at 350°C in an air atmosphere, and the sintering time is 10h , after natural cooling, take it out from the crucible or other heating reaction device; smash it again and mix it evenly, transfer it to the crucible or other heating reaction device and put it into a muffle furnace, and sinter at 1400 ° C for 2 hours under air atmosphere to obtain the solid After natural cooling and grinding, it becomes yellow phosphor Bi 0.99 Ca 3 (PO 4 ) 3 O:0.01Dy 3+ . The pu...
Embodiment 2
[0050] A kind of fluorescent powder, its chemical formula is: Bi 1-x Ca 3 (PO 4 ) 3 O:xDy 3+ , where x=0.03. The above-mentioned phosphor Bi 0.97 Ca 3 (PO 4 ) 3 O:0.03Dy 3+ The preparation method:
[0051] Weigh CaCO 3 : 3g, Bi 2 o 3 : 226g, NH 4 h 2 PO 4 : 3.451g, Dy 2 o 3 : 5.595g. Put the above compound into a quartz mortar and crush it by grinding and mixing evenly, then transfer it to a crucible or other heating reaction device and place it in a muffle furnace, and pre-sinter at 500°C in an air atmosphere for 10 hours. , after natural cooling, take it out from the crucible or other heating reaction device; pulverize again and mix evenly, transfer to the crucible or other heating reaction device and put it into the muffle furnace, and sinter at 1000 ° C for 10 h under the condition of air atmosphere to obtain the solid After natural cooling and grinding, it becomes yellow phosphor Bi 0.97 Ca 3 (PO 4 ) 3 O:0.03Dy 3+ .
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