Thiadizole dimer additives and lubricating compositions containing the same
A technology of thiadiazole dimer and lubricating composition is applied in the field of thiadiazole dimer additive and lubricating composition containing the additive, and can solve problems such as poor Timken load performance and the like
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Embodiment 1
[0039] The reaction product of thiadiazole dimer-diol is synthesized like this: add 112.9 g of DMTD disulfide dimers (5,5'-dithiobis(1,3,4-thiabis) in a three-necked flask Azole-2-thiol) (i.e., a compound of formula (I) wherein Z is hydrogen ("H") and n is 2) and 138.6 g of butoxytriethylene glycol yielded a molar ratio of 0.53:1 Reaction raw material. DMTD disulfide dimer can trade name VANLUBE 829 is commercially available from R.T. Vanderbilt, Company, Inc. The mixture, which did not contain any other reactants, was heated at 135°C for 1 hour. After cooling the mixture, unreacted solid starting material (ie, DMTD disulfide dimer) was removed from the liquid reaction product by filtration. The structural features of the liquid reaction product (Compound 1) are listed in Table 1.
Embodiment 2-4
[0041] Following the general procedure described in Example 1, the DMTD disulfide-dipolymer of Example 1 was mixed with a poly(ether)diol having the structure of formula (III) at the specified molar ratios to prepare thiadiazole dimers -Reaction products of diols. The substituent "Z" can be hydrogen or an alkoxy chain having the structure of formula (II). As in Example 1, the reaction mixture was heated to at least 100°C for at least 30 minutes. After cooling the mixture, the liquid reaction product was filtered to remove unreacted thiadiazole dimer starting material. The structural features of the reaction product (compound 2-4) are shown in Table 1 below.
Embodiment 5
[0043] The thiadiazole dimer-diol reaction product was synthesized by using DMTD instead of DMTD dimer. Approximately 16.3 g of DMTD, 21.2 g of triethylene glycol, and 0.14 g of aluminum trichloride were added to the round bottom flask. The flask was connected to a scrubber containing sodium hydroxide to remove hydrogen sulfide during in situ dimer formation. The mixture was heated at 115–145 °C for 6 h, during which, the evolution of H was observed 2 S, indicating the in situ formation of DMTD dimers. After cooling the reaction mixture, unreacted starting material was removed by filtration. The structural features of the reaction product (compound 5) are shown in Table 1 below.
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