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High silicon mordenite and preparing method thereof

A mordenite and high-silicon technology, which is applied in the field of high-silicon mordenite and its preparation, can solve the problems of high benzene adsorption value, no mention of the preparation method of high-silicon mordenite with low benzene adsorption value, etc., and achieves the effect of low production cost.

Inactive Publication Date: 2004-04-21
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0008] One of the technical problems to be solved by the present invention is the problem that the benzene adsorption value of the prepared mordenite exists in the previous literature, and a new high-silica mordenite is provided.
[0009] The second technical problem to be solved by the present invention is that the preparation method of high-silica mordenite with low benzene adsorption value has not been mentioned in previous documents, and a new preparation method of high-silica mordenite is provided

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] 213.7 g silica sol [40, SiO 2 % (weight), all the other are water, the same below] is A solution, 81.0 grams of solid aluminum sulfate [chemically pure, Al 2 (SO 4 ) 3 18H 2 O, the same below] was dissolved in 140 milliliters of water to obtain solution B, and 54.5 grams of solid sodium hydroxide (chemically pure) was dissolved in 113 milliliters of water to obtain solution C. Add 200 ml of water into a container with a stirring device, turn on the stirring device, and add the three solutions of A, B, and C into the container at the same time in proportion to the flow, within 45 to 90 minutes, the three solutions are added at the same time, and continue to stir for 15 minutes Above, add 8.3 grams of ammonia water [chemically pure, NH 3 25.5% (weight)], and then stirred for 1 to 3 minutes. Then transfer the slurry into a 2-liter crystallization tank with a stirring device, seal the crystallization tank, turn on the stirring device, start heating, raise the temperatu...

Embodiment 2

[0023] 230.4 grams of silica sol was solution A, 51.1 grams of solid aluminum sulfate was dissolved in 191 milliliters of water to obtain solution B, and 33.2 grams of solid sodium hydroxide was dissolved in 120 milliliters of water to obtain solution C. Add 380 ml of water into a container with a stirring device, turn on the stirring device, and add the three solutions of A, B, and C into the container at the same time in proportion, and continue stirring for more than 15 minutes after adding the three solutions at the same time, then add 5.1 grams Ammonia [chemically pure, NH 3 25.5% (weight)], and then stirred for 1 to 3 minutes. Then transfer the slurry into a 2-liter crystallization tank with a stirring device, seal the crystallization tank, raise the temperature in the crystallization tank to 180° C. within 2 hours, and keep the temperature constant for 28 hours. Then cool, filter and recover the solid product, wash with water, and dry overnight at 110°C to obtain the s...

Embodiment 3

[0028] 239.4 grams of industrial water glass (26.02% by weight SiO 2 , 7.45 wt% Na 2 (2, all the other being water) is A solution, and 41.6 grams of solid aluminum sulfate and 17.8 grams of sulfuric acid (chemically pure) are dissolved in 228 milliliters of water to obtain B solution. Add 300 ml of water into a container with a stirring device, turn on the stirring device, and add the two solutions of A and B into the container at the same time in proportion to the parallel flow. After the two solutions are added at the same time, continue to stir for more than 15 minutes, and then transfer the slurry into 2 Lift the crystallization kettle with a stirring device, seal the crystallization kettle, then bubble 3.2 grams of liquid ammonia (purity above 99%) into the crystallization kettle, raise the temperature in the crystallization kettle to 170°C, and keep the constant temperature at 60°C Hour. Then cool, filter and recover the solid product, wash with water, and dry overnigh...

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Abstract

A high-Si mordenite with high absorbtivity to benzene is prepared from water glass or silicon sol or silica gel as Si source, aluminium salt or aluminate as Al source, inorganic acid and inorganic alkali through proportioning, reacting under existance of ammonia, and crystallizing at 120-250 deg.C for 4-400 hr.

Description

technical field [0001] The invention relates to a high-silicon mordenite and a preparation method thereof, in particular to a directly synthesized high-silicon mordenite and a preparation method thereof. Background technique [0002] Mordenite is widely used as an adsorbent for separating gas or liquid mixtures, and as a catalyst carrier and catalyst in chemical and petrochemical industries, such as disproportionation, isomerization, alkylation, transalkylation of aromatics, disproportionation of alkanes, iso Structuralization, esterification, etherification, amination and other reactions of alcohols. Mordenite is a new type of catalytic material that attracts people's attention. [0003] Mordenite, regardless of natural mordenite and mordenite synthesized by general methods, its silicon-aluminum ratio (SiO 2 / Al 2 o 3 Molar ratio) is 10~12. However, some catalytic reaction processes require mordenite with a higher silicon-aluminum ratio as a...

Claims

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Application Information

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IPC IPC(8): C01B39/00C01B39/02C01B39/26
Inventor 程文才杨德琴孔德金李华英朱志荣
Owner CHINA PETROLEUM & CHEM CORP