Copolymer based on oxidative olefinic diols alkenyl ether and unsaturated dicarboxylic acid derivatives
A technology of oxyalkylene glycol alkenyl ether and dicarboxylic acid derivatives, which is applied in the field of additives to improve the performance of building materials produced therefrom during processing and solidification, and can solve the problems of reduced strength and stability of hardened building materials.
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Embodiment 1
[0096] 270 g of water were placed in a reaction vessel equipped with a thermometer, a stirrer, a reflux condenser and two connecting pipes respectively connected to the inlets. While stirring, 32.7 g (0.334 mol) of maleic anhydride and 25.0 g of a 50% aqueous sodium hydroxide solution were added thereto, and the temperature thereof was kept below 30° C. by cooling. Subsequently, while stirring, 100 mg of ferric sulfate heptahydrate and 18.5 g of 30% hydrogen peroxide from the respective supply container were added thereto, on the one hand, a solution of 5.1 g of sodium hydroxymethanesulfinate dihydrate and 12.5 g of water (Raw material 1) was added thereto during 75 minutes, on the other hand, 155 g (0.310 mol) of methyl polyethylene glycol monovinyl ether (molecular weight 500) and 12.1 g (0.006 mol) of polypropylene glycol dimalemic acid ( A solution of molecular weight 2000) (raw material 2) was added during 60 minutes.
[0097] After the addition was complete, stirring wa...
Embodiment 2
[0099] The procedure was as described in Example 1, but using the following vinyl ether feedstock composition (feedstock 2):
[0100] 155.0g (0.310mol) methyl polyethylene glycol monovinyl ether (molecular weight 500)
[0101] 7.4g (0.001mol) polydimethylsiloxane-bis-(dipropylene aminomaleamic acid) (molecular weight 5400)
[0102] At the end of the addition, the reaction mixture had a pH of 5.02 and was subsequently neutralized with 20% aqueous sodium hydroxide (58.3 g). The solids content in the final product was 35.5% by weight.
Embodiment 3
[0104] Example 1 was repeated using feedstock 2 with the following composition:
[0105] 116.0g (0.232mol) methyl polyethylene glycol monovinyl ether (molecular weight 500)
[0106] 9.1g (0.0875mol) styrene
[0107] 5.2g (0.0026mol) polypropylene glycol dimalemic acid (molecular weight 2000)
[0108] The water-dispersed reaction product after neutralization with a 20% aqueous sodium hydroxide solution had no residual monomer styrene and had a solid content of 33.7% by weight.
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