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High stability color-less rosin pentaerythrite ester and its prepn

A rosin pentaerythritol ester and high-stability technology, which is applied in the field of high-stability colorless rosin pentaerythritol ester and its preparation, can solve the problems such as the color, thermal stability and weather resistance of rosin esterified products cannot meet the higher requirements of esterified products. , to achieve the effect of good thermal stability and weather resistance, complex production process and light color of the product

Inactive Publication Date: 2008-01-02
INST OF CHEM IND OF FOREST PROD CHINESE ACAD OF FORESTRY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The third method is to obtain light-colored rosin esters by adding a decolorizing agent, such as JP9143430, JP8209070, US5504152, US 5387669, US 5387669, WO0006657, etc. have invented the addition of organic phosphorus with decolorization during the esterification process or after the esterification is completed. However, the rosin esters obtained by these methods still cannot meet people's higher requirements for esterified products in terms of color, thermal stability, and weather resistance.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] A high-stability colorless rosin pentaerythritol ester, the resin has a Hasson color number less than 150; good thermal stability: placed in a blast drying oven at 180°C for 8 hours, the color change is not more than 1 Ghanaian color number; weather resistance Good: 15h at 20°C and 50cm away from 500W UV lamp, the weight gain rate is not more than 0.2%, and the color change is not more than 3 Ghanaian colors.

Embodiment 2

[0025] A method for preparing high-stability colorless rosin pentaerythritol ester, including the following steps:

[0026] In the first step, the super-grade rosin is distilled at a vacuum of 0~1kPa and a temperature of 180~270℃. The Ghana color number of the color produced is no greater than No. 3, the acid value is 160mg / g~190mg / g, and the softening point is 70℃. ~85℃ refined rosin;

[0027] In the second step, in an inert atmosphere, the inert atmosphere can be N 2 , Ar, He, CO 2 In the refined rosin, add pentaerythritol which accounts for 11.0-16.0% of the refined rosin mass, a decolorant which accounts for 0.1-1.0% of the refined rosin mass, and anthraquinone as an antioxidant which accounts for 0.01-0.1% of the refined rosin mass. A catalyst with 0.1% to 0.5% rosin mass is used for esterification at 230 to 290°C. The reaction is 3-10 hours, and the reaction is completed until the acid value is less than 20mg / g; among them, the decolorizing agent is 4,4-thiobis- (6-tert-buty...

Embodiment 3

[0033] Add 1000g refined rosin, 140g pentaerythritol, 2g 300, 0.2g anthraquinone, 3g ZnO into the reaction flask, and pass N 2 , Heat to 280±2℃, react until the acid value is less than 20mg / g, reduce pressure, keep the vacuum degree at 0~0.6kPa until there is no distillate, reduce the temperature to 220℃, add 1g 2,6-di-tert-butyl- 4-methylphenol, 1 g of tris(nonylphenyl phosphite) and 1 g of 2-hydroxy-4-n-octyloxybenzophenone.

[0034] The product in this example (colorless rosin pentaerythritol ester 1) color: 150 (Hasson color number), acid value: 14.2 mg / g, softening point: 105.1°C, thermal stability test (180°C, 8h): color, 200 (Hassen color number); weather resistance test: weight gain rate, 0.20%, color increased by 3 Ghana color numbers.

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Abstract

The present invention discloses one kind of high stability color-less rosin pentaerythrite ester with Hason color number smaller than 150, color change after being set in a drying tank at 180 deg.c for 8 hr not greater than 1 Ghana color number and color change after being irradiated with ultraviolet lamp for 15 hr not greater than 3 Ghana color number. Its preparation process includes the following steps: distilling rosin to obtain refined rosin; adding pentaerythritol, decolorizing agent, antioxidant and catalyst to refined rosin for esterification until reaching acid value lower than 20 mg / g; decompressing to eliminate low boiling point matter; cooling, adding heat stabilizer and light stabilizer via stirring to obtain the high stability color-less rosin pentaerythrite ester. The present invention has simple technological process and low production cost.

Description

Technical field [0001] The invention relates to a rosin pentaerythritol ester and a preparation method thereof, in particular to a high-stability colorless rosin pentaerythritol ester and a preparation method thereof. Background technique [0002] Rosin ester is a deep-processed product of rosin obtained by the reaction of rosin and polyol, and has a history of more than 70 years. It has a wide range of uses, and can be used as a tackifier for packaging materials, pressure-sensitive adhesives, hot melt adhesives, etc., a modifier for rubber and plastics, and a setting agent for cosmetics. [0003] In many applications, the color and stability of rosin ester is an important indicator that determines its market viability. Since the 1970s, a lot of research has been done on the production of light-colored rosin and its esters at home and abroad. There are about two methods: The method represented by US Patent 5,395,920 is to obtain colorless rosin ester by...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09F1/04
Inventor 高宏宋湛谦商士斌王振洪饶小平
Owner INST OF CHEM IND OF FOREST PROD CHINESE ACAD OF FORESTRY