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Catalyst for selective catalytic reduction denitration of steam electric plant and preparation method thereof

A catalyst and selective technology, applied in the direction of physical/chemical process catalysts, chemical instruments and methods, metal/metal oxide/metal hydroxide catalysts, etc., can solve the problems of low catalyst use temperature, catalyst poisoning and deactivation, and catalyst coking Inactivation and other problems, to achieve high dispersion, slow down poisoning inactivation, reduce the effect of dosage

Active Publication Date: 2013-04-24
京能科技(易县)有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] (1) Pd / Pt catalyst and SO 2 / SO 3 reaction, causing the catalyst to be quickly poisoned and deactivated when used;
[0007] (2) The use temperature of Pd / Pt catalysts is low, generally at 200-300°C, but the temperature may reach above 300°C in actual application, which will lead to coking and deactivation of the catalyst;
[0008] (3) The amount of precious metals is large and expensive
[0012] (1)V 2 o 5 Easy to remove SO from flue gas 2 Oxidation to SO 3 , SO 3 with escaped NH 3 , The water vapor in the flue gas reacts to form ammonium bisulfate, which is highly viscous and will deposit on the heating surface, while the SCR catalyst is generally installed upstream of the air preheater. Ammonium bisulfate is most likely to cause blockage and corrosion of the equipment and pipelines;

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0031] This embodiment provides a catalyst for selective catalytic reduction and denitrification in thermal power plants, which is prepared according to the following specific steps:

[0032] (1) Dissolve 30g of urea in water to make a urea solution with a concentration of 1mol / L, and place it in an airtight corrosion-resistant container for use; 300g of corrugated γ-Al 2 o 3 The carrier was added to the urea solution, the temperature was raised to 80°C, and then stirred at a speed of 50r / min for 8 hours (in order to prevent the urea from decomposing and volatilizing during the stirring process, the container was sealed), then naturally cooled to room temperature, and the γ- al 2 o 3carrier, and the carrier was washed several times with desalted water to obtain surface-activated γ-Al 2 o 3 carrier;

[0033] (2) Dissolve 100g of ferric nitrate in 100mL of demineralized water to make a ferric nitrate solution, and the activated γ-Al 2 o 3 Put the carrier into the ferric n...

Embodiment 2

[0044] This embodiment provides a catalyst for selective catalytic reduction and denitrification in thermal power plants, which is prepared according to the following specific steps:

[0045] (1) Dissolve 20g of urea in water to make a urea solution with a concentration of 0.8mol / L, and place it in a sealable corrosion-resistant container for use; 2 o 3 Add the carrier into the urea solution, raise the temperature to 90°C, and stir at a speed of 100r / min for 6 hours (in order to prevent the urea from decomposing and volatilizing during the stirring process, the container is sealed), naturally cool to room temperature, and filter out the γ-Al 2 o 3 carrier, and the carrier was washed several times with desalted water to obtain surface-activated γ-Al 2 o 3 carrier.

[0046] (2) Dissolve 150g of ferric nitrate in 100mL of demineralized water to make a ferric nitrate solution, and the activated γ-Al 2 o 3 The carrier was added to the ferric nitrate solution, stirred at 70°C ...

Embodiment 3

[0057] This embodiment provides a catalyst for selective catalytic reduction and denitrification in thermal power plants, which is prepared according to the following specific steps:

[0058] (1) Dissolve 30g of urea in water to make a urea solution with a concentration of 1.5mol / L, and place it in an airtight corrosion-resistant container for use; 300g of corrugated γ-Al 2 o 3 The carrier was added to the urea solution, heated to 80°C, stirred at a speed of 70r / min for 8 hours, naturally cooled to room temperature, and γ-Al was filtered out 2 o 3 carrier, and the carrier was washed several times with desalted water to obtain surface-activated γ-Al 2 o 3 carrier.

[0059] (2) Dissolve 120g of ferric nitrate in 100mL of demineralized water to make a ferric nitrate solution, and the activated γ-Al 2 o 3 The carrier was put into the ferric nitrate solution, stirred at 70°C for 8 hours, then cooled and the prepared catalyst precursor was washed, then placed in a desiccator, ...

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PUM

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Abstract

The invention relates to a catalyst for selective catalytic reduction denitration of a steam electric plant and a preparation method of the catalyst. The catalyst is characterized in that vanadium, tungsten, and molybdenum are main catalytical metals, iron is utilized as an assisting catalytical metal, and gamma-Al2O3 is utilized as a carrier. The catalyst comprises the chemical composition of VxWyMozFemOn / Al2O3, wherein x=0.0.1-0.10, y=0.01-0.20, z=0.01-0.20, m=0.01-0.50, and n=0.05-1.50. The invention also provides the preparation method of the catalyst. The catalyst provided by the invention has high tolerable temperature and hardly causes a reactive metal sintering phenomenon, the noble metal dosage is low, and the manufacturing cost is low.

Description

technical field [0001] The invention relates to a catalyst for selective catalytic reduction denitration in a thermal power plant and a preparation method thereof, belonging to the technical field of catalyst preparation for denitration. Background technique [0002] The main pollutants in the flue gas emitted by thermal power plants include sulfur dioxide, nitrogen oxides and dust. After desulfurization and dust removal have reached a certain scale, denitrification will undoubtedly become the next hot spot in the field of environmental protection according to the new standard of thermal power sewage discharge. [0003] The newly revised "Emission Standards of Air Pollutants for Thermal Power Plants" came into effect in 2012. Among them, from January 1, 2012, the emission limit of nitrogen oxides (calculated as nitrogen dioxide) for newly built thermal power units is 100 mg / m3; Except for the emission limit of 200 mg / m3, the rest are required to meet the standard of not hi...

Claims

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Application Information

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IPC IPC(8): B01J23/888B01D53/90B01D53/56
Inventor 陈鹏贾向东王力彪刘玉龙陈海文刘超赵岩孙翠霞
Owner 京能科技(易县)有限公司