Preparation method of anhydrous ammonium bifluoride and microchannel reaction device thereof
An anhydrous hydrogen fluoride, microchannel reaction technology, applied in chemical instruments and methods, ammonium halide, chemical/physical processes, etc., can solve the problems of large working environment pollution, complex equipment structure, waste of raw materials, etc., and achieve low labor intensity, The effect of small size and no material waste
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[0031] The preparation method of anhydrous ammonium bifluoride of the present invention, wherein reaction raw material hydrogen fluoride and liquid ammonia are all in liquid phase; Reaction is carried out in two steps: the first step first liquid phase reaction, takes away most of reaction heat; The second step utilizes reaction heat, From the liquid phase reaction to the molten state; after cooling, anhydrous ammonium bifluoride is obtained. The adopted scheme is: a) React liquid hydrogen fluoride and liquid ammonia in the microchannel reactor in the heat exchange section of the microchannel reaction device to obtain a solution of ammonium bifluoride and hydrogen fluoride; the temperature of the microchannel reactor in the heat exchange section during the above reaction process Less than or equal to 90°C; (b) Input the solution of ammonium bifluoride and hydrogen fluoride obtained in step (a) into the microchannel reactor in the melting section, continue to feed liquid ammonia...
Embodiment 1
[0037] A kind of preparation method of anhydrous ammonium bifluoride, comprising: see attached figure 2 as shown,
[0038] a) Pass 710g of liquid hydrogen fluoride and 200g of liquid ammonia into the microchannel reactor in the heat exchange section of the microchannel reaction device to react to obtain a solution of ammonium bifluoride and hydrogen fluoride; wherein, the flow rate of hydrogen fluoride is 35-36g / min, and the liquid The flow rate of ammonia is 10-11g / min. During the above reaction process, the temperature of the microchannel reactor in the heat exchange section is controlled at 80-90° C. by circulating cooling water;
[0039] (b) Input the solution of ammonium bifluoride and hydrogen fluoride obtained in step (a) into the microchannel reactor in the melting section, continue to feed 103g of liquid ammonia, and the flow rate of liquid ammonia is 10-11g / min. React to obtain ammonium bifluoride in a molten state; during the reaction process, the temperature of ...
Embodiment 2
[0043] A kind of preparation method of anhydrous ammonium bifluoride, comprising: see attached figure 2 as shown,
[0044]a) Pass 750g of liquid hydrogen fluoride and 210g of liquid ammonia into the microchannel reactor in the heat exchange section of the microchannel reaction device to react to obtain a solution of ammonium bifluoride and hydrogen fluoride; wherein, the flow rate of hydrogen fluoride is 35-36g / min, and the liquid The flow rate of ammonia is 10-11g / min. During the above reaction process, the temperature of the microchannel reactor in the heat exchange section is controlled at 65-70° C. by circulating cooling water;
[0045] (b) Input the solution of ammonium bifluoride and hydrogen fluoride obtained in step (a) into the microchannel reactor in the melting section, continue to feed 120g of liquid ammonia, and the flow rate of liquid ammonia is 10-11g / min. React to obtain ammonium bifluoride in a molten state; during the reaction process, the temperature of t...
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