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A kind of silicon negative electrode lithium-ion battery and manufacturing method thereof

A technology for a lithium ion battery and a manufacturing method, applied in the field of lithium ion batteries, can solve the problems of short cycle life and low specific capacity, and achieve the effects of excellent charge and discharge performance, high battery energy density and low price

Active Publication Date: 2016-08-31
NINGBO VEKEN BATTERY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The disadvantage is that the cycle life is short and the specific capacity is low

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0028] A silicon negative electrode lithium-ion battery, comprising a positive electrode, a negative electrode and a diaphragm between the positive and negative electrodes, the silicon negative electrode lithium-ion battery is a laminated structure, and the negative electrode is composed of a current collector, an active material, a conductive agent and a bonding agent. The active material is a silicon-carbon composite material coated with a carbon layer, and the carbon layer is formed by pyrolysis of starch. The active substance is prepared through the following steps:

[0029] Step a) Ball milling: 1000g of natural graphite powder and 500g of silicon powder with a particle size of 40 microns were mechanically milled for 4 hours in an argon atmosphere with a ball milling speed of 100rpm to obtain a silicon-carbon composite material, wherein the vibration of the natural graphite powder The density is 0.96g / c㎡;

[0030] Step b) Dissolving and stirring: dissolving 600g of starc...

Embodiment 2

[0035] A silicon negative electrode lithium-ion battery, comprising a positive electrode, a negative electrode and a diaphragm between the positive and negative electrodes, the silicon negative electrode lithium-ion battery is a laminated structure, and the negative electrode is composed of a current collector, an active material, a conductive agent and a bonding agent. The active substance is a silicon-carbon composite material coated with a carbon layer, and the carbon layer is formed by pyrolysis of lactose.

[0036] The active substance is prepared through the following steps:

[0037] Step a) Ball milling: 1500g of activated carbon and 500g of silicon powder with a particle size of 50 microns were mechanically milled with high-energy ball in an argon atmosphere for 5 hours, and the milling speed was 400rpm to obtain a silicon-carbon composite material, wherein the tap density of natural graphite powder was 0.96g / c㎡;

[0038] Step b) Dissolving and stirring: Dissolve 800g...

Embodiment 3

[0043] A silicon negative electrode lithium-ion battery, comprising a positive electrode, a negative electrode and a diaphragm between the positive and negative electrodes, the silicon negative electrode lithium-ion battery is a laminated structure, and the negative electrode is composed of a current collector, an active material, a conductive agent and a bonding agent. The active material is a silicon-carbon composite material coated with a carbon layer, and the carbon layer is formed by pyrolysis of dextrin. The active substance is prepared through the following steps:

[0044] Step a) Ball milling: 2500g of natural graphite powder and 500g of silicon powder with a particle size of 30 microns were mechanically milled with high-energy ball for 7 hours in an argon atmosphere to obtain a silicon-carbon composite material, wherein the tap density of the natural graphite powder was 0.96g / c㎡;

[0045] Step b) Dissolving and stirring: Dissolving 1000g of sucrose in 15000g of dist...

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Abstract

The invention relates to a silicon negative electrode lithium ion battery with high specific capacity and good cycle performance and a manufacturing method thereof. It includes a positive electrode, a negative electrode, and a diaphragm between the positive and negative electrodes. The silicon negative electrode lithium-ion battery is a laminated structure. The negative electrode includes a current collector, an active material, a conductive agent, and a binder. The active material is carbon Layer-coated silicon-carbon composites. Using the silicon-carbon composite material of the invention as the negative electrode has the advantages of high battery energy density, safety and reliability, and low price compared with the graphite negative electrode material; and the charging and discharging performance is excellent.

Description

technical field [0001] The invention relates to the field of lithium ion batteries, in particular to a silicon negative electrode lithium ion battery and a manufacturing method thereof. Background technique [0002] With the rapid development of electric vehicles and hybrid electric vehicles, there is a demand for power lithium-ion batteries with higher power density and energy density, suitable for fast charging and discharging, and energy-type lithium-ion batteries with longer battery life very urgent. The main idea of ​​developing a lithium-ion battery that meets the above requirements is to find new positive and negative electrode materials, so that the battery has a higher lithium intercalation capacity and good delithiation reversibility, so as to ensure the high voltage, large capacity and long cycle life of the battery . The current commercial lithium-ion battery negative electrode uses graphite-based materials, which have the advantages of preventing lithium dendr...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01M10/0525H01M4/38H01M4/583H01M4/62H01M4/134H01M10/0585
CPCH01M4/364H01M4/386H01M4/587H01M10/0525H01M10/0585Y02E60/10Y02P70/50
Inventor 曹长河潘美姿刘旭
Owner NINGBO VEKEN BATTERY