A kind of superhydrophobic coating and preparation method thereof
A technology of super-hydrophobic coatings and nanomaterials, applied in the field of super-hydrophobic coatings and its preparation, can solve problems such as poor hydrophobicity, and achieve good compatibility, good hydrophobicity, and controllable molecular structure and composition
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Embodiment 1
[0030] Embodiment 1: the molecular weight of fluorine-containing block copolymer is 10000, and the structure is:
[0031]
[0032] Wherein, m=13, n=50.
[0033] A. Preparation of fluorine-containing block copolymers
[0034] Add 15.7 g of 2-(N,N-dimethylamino)ethyl methacrylate (DMAEMA), 0.3880 g of α-bromoisobutyrate (EBiB) and 0.3880 g of CuBr into a 500 ml four-necked flask. 2 0.0183g, pentamethyldiethylenetriamine (PMDETA) 0.1301g, stannous octoate Sn(EH) 2 0.3038g, solvent toluene 7.85g, after mixing uniformly, nitrogen gas was passed for 2h, and reacted in an oil bath at 80°C for 5h. After the conversion rate reached 85%, a light yellow viscous product was obtained. Then, 4.2 g of trifluoroethyl methacrylate (TFEMA) was added into the reaction vessel, and the reaction was continued for 4 hours. After the reaction, a yellow viscous substance, namely a fluorine-containing block copolymer, was obtained.
[0035] B. Preparation of Superhydrophobic Coatings
[0036] 1....
Embodiment 2
[0042] Embodiment 2: the molecular weight of fluorine-containing block copolymer is 12000, and the structure is:
[0043]
[0044] Wherein, m=10, n=60.
[0045] A. Preparation of fluorine-containing block copolymers
[0046] Add DMAEMA 15.7g, EBiB 0.3232g, CuBr 2 0.0122g, PMDETA0.08675g, Sn(EH) 2 0.3038g, 7.85g of toluene, after mixing evenly, after passing nitrogen for 2 hours, reacting in an oil bath at 80°C for 5 hours, the conversion rate reached 83%, and a light yellow viscous product was obtained. Then, 4.1667 g of hexafluorobutyl methacrylate (HFBMA) was added into the reaction vessel, and the reaction was continued for 4 hours. After the reaction, a yellow viscous substance, namely a fluorine-containing block copolymer, was obtained.
[0047] B. Preparation of Superhydrophobic Coatings
[0048] 1. 2-(N,N-dimethylamino)ethyl methacrylate-b-polyhexafluorobutyl methacrylate block copolymer / nano-CaCO 3 Preparation of hybrid materials
[0049] The fluorine-containi...
Embodiment 3
[0054] Embodiment 3: the molecular weight of fluorine-containing block copolymer is 12000, and the structure is:
[0055]
[0056] Wherein, m=6, n=60.
[0057] A. Preparation of fluorine-containing block copolymers
[0058] Add DMAEMA15.7g, EBiB 0.3232g, CuBr 2 0.0244g, PMDETA0.1733g, Sn(EH) 2 0.6076g, 7.85g of toluene, mixed evenly, nitrogen gas for 2h, reacted in 80°C oil bath for 5h, the conversion rate reached 86%, and a light yellow viscous product was obtained. Then, 4.0 g of dodecafluoroheptyl methacrylate (DFHMA) was added into the reaction vessel, and the reaction was continued for 4 hours. After the reaction, a yellow viscous substance, namely a fluorine-containing block copolymer, was obtained.
[0059] B. Preparation of Superhydrophobic Coatings
[0060] 1. N, N-dimethylaminoethyl methacrylate-b-polydodecafluoroheptyl methacrylate block copolymer / nano-TiO 2 Preparation of hybrid materials
[0061] The fluorine-containing block copolymer obtained in step A ...
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