A preparation method of flame-retardant heat-resistant polyphosphazene insulating glue
A technology of polyphosphazene and insulating glue is applied in the field of wire and cable materials, which can solve the problems of limited high temperature resistance and poor thermal stability, and achieve the effects of improving water resistance, excellent electrical insulation performance and improving stability.
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Embodiment 1
[0059] A preparation method of flame-retardant heat-resistant polyphosphazene insulating glue, comprising the following steps:
[0060] Step 1. Take 58g of polyphosphazene chloride, add it to 400mL tetrahydrofuran solution, and stir until the polyphosphazene chloride is completely dissolved to obtain a tetrahydrofuran solution of polyphosphazene chloride, which is set aside;
[0061] Step 2: Dissolve 130.1g of 2,6-difluorophenol in 150mL of tetrahydrofuran solution, slowly add 40g of sodium hydroxide through a stirrer, adjust the temperature of the solution to a constant temperature of 40°C, and react under stirring for 1 hour to 2,6 - until the complete reaction of difluorophenol is sodium difluorophenoxide, the intermediate product solution (I) is obtained, and it is subsequent use;
[0062] Step 3: Take a 1000mL three-neck flask equipped with a stirrer, condenser and constant pressure dropping funnel, add 33.2g of 1,7-bis(4-hydroxyphenyl)-carborane, and slowly add 4g of hyd...
Embodiment 2
[0068] The difference between embodiment two and embodiment one is:
[0069] In step 2, get 162.1g p-trifluoromethylphenol and dissolve in 150mL tetrahydrofuran solution, and react under stirring for 1 hour until p-trifluoromethylphenol is completely reacted as p-trifluoromethylphenoxysodium to obtain the intermediate product Solution (Ⅱ), standby;
[0070] In step 3, when passing nitrogen into the reaction solution, the stirring reaction was carried out at a temperature of 100° C. for 2 hours;
[0071] In step 4, the intermediate product solution (II) is used for the reaction.
[0072] The beneficial effects of the present invention are: the water resistance of polyphosphazene is improved by replacing the chlorine atom of polydichlorophosphazene polymer with alkoxy group, but the thermal stability is not good, and carborane is added in the substituent, then improved Polyphosphazene polymer stability, heat resistance. The electrical cable insulating adhesive prepared by add...
Embodiment 3
[0074] The difference between embodiment three and embodiment one is:
[0075] In step 2, get 178.1g p-trifluoromethoxyphenol and dissolve in 150mL tetrahydrofuran solution, react under stirring for 1 hour until p-trifluoromethoxyphenol is completely reacted as p-trifluoromethylphenoxysodium, to obtain Intermediate product solution (Ⅲ), standby;
[0076] In step 3, when passing nitrogen into the reaction solution, the stirring reaction was carried out at a temperature of 100° C. for 2 hours;
[0077] In step 4, the intermediate product solution (III) is used for the reaction.
[0078] The beneficial effects of the present invention are: the water resistance of polyphosphazene is improved by replacing the chlorine atom of polydichlorophosphazene polymer with alkoxy group, but the thermal stability is not good, and carborane is added in the substituent, then improved Polyphosphazene polymer stability, heat resistance. The electrical cable insulating adhesive prepared by addin...
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