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Preparation method of alkyl glycoside of asymmetric Gemini structure

An alkyl glycoside, asymmetric technology, applied in the field of preparation of asymmetric Gemini structure alkyl glycosides, can solve the problems of heavy environmental pollution, difficult rinsing, and the modification of alkyl glycosides can not significantly improve the surface properties, etc., to achieve safe and reliable process , Good product quality and low production cost

Inactive Publication Date: 2016-11-09
郭迎庆
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The technical problem mainly solved by the present invention: Aiming at the problem that the alkyl glycoside aqueous solution has rich foam, is not easy to rinse, and has great environmental pollution, and the modification of the alkyl glycoside cannot significantly improve its surface performance, this method provides a new type of non-toxic The preparation method of symmetrical alkyl glucoside; the present invention uses tapioca starch as raw material to directly prepare starch-based dodecyl glucoside, which is substituted and quaternized with hexadecyldimethyl tertiary amine and epichlorohydrin to synthesize asymmetric Gemini structure alkyl glycoside surfactant; the asymmetric Gemini structure alkyl glycoside prepared by the present invention has both the greenness of the alkyl glycoside and the high efficiency of the asymmetric Gemini structure, and has excellent foam performance and emulsification performance, and wettability good

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0017] First weigh 60g of tapioca starch, add it to 100mL of ethylene glycol, stir at 300r / min for 15min, slowly add 5mL of sulfuric acid solution with a mass concentration of 98%, continue stirring for 30min, add 80g of n-dodecyl alcohol, and add 1.6g of p-toluenesulfonic acid , heated to 115°C, reacted for 4h, cooled to 75°C, stood still for 2h, adjusted the pH to 8 with a mass fraction of 1% sodium hydroxide solution, and distilled under reduced pressure to obtain starch-based dodecyl glucoside for later use; then weighed Take 80g of hexadecyldimethyl tertiary amine hydrochloride, add it to 80mL of absolute ethanol, stir at 300r / min for 15min, add 10mL of epichlorohydrin dropwise at 0.5mL / min to the mixture, and keep the temperature at 25°C Under a water bath, react for 3 hours, distill under reduced pressure to 30% of the volume of the original solution, and filter with suction to obtain a white needle-like solid; then weigh 50 g of the starch-based dodecyl glucoside prepar...

example 2

[0020] First weigh 70g of tapioca starch, add it to 110mL of ethylene glycol, stir at 350r / min for 18min, slowly add 7mL of sulfuric acid solution with a mass concentration of 98%, continue stirring for 35min, add 90g of n-dodecyl alcohol, add 1.8g of p-toluenesulfonic acid , heated to 118°C, reacted for 4.5h, cooled to 78°C, stood still for 2.5h, adjusted the pH to 8.5 with a mass fraction of 1% sodium hydroxide solution, and distilled under reduced pressure to obtain starch-based dodecyl glucoside for later use; Then weigh 85g of hexadecyl dimethyl tertiary amine hydrochloride, add it into 90mL of absolute ethanol, stir at 350r / min for 18min, add 11mL of epichlorohydrin dropwise to the mixed solution at 0.5mL / min, at 25 ~30°C constant temperature water bath, react for 3.5h, distill under reduced pressure to 35% of the volume of the original solution, and filter with suction to obtain a white needle-like solid; then weigh 55g of the starch-based dodecyl glucoside prepared by t...

example 3

[0023]First weigh 80g of tapioca starch, add it to 120mL of ethylene glycol, stir at 400r / min for 20min, slowly add 8mL of sulfuric acid solution with a mass concentration of 98%, continue stirring for 40min, add 100g of n-dodecyl alcohol, and add 2.0g of p-toluenesulfonic acid , heated to 120°C, reacted for 5h, cooled to 80°C, stood still for 3h, adjusted the pH to 9 with a mass fraction of 1% sodium hydroxide solution, and distilled under reduced pressure to obtain starch-based dodecyl glucoside for later use; then weighed Take 90g of hexadecyldimethyl tertiary amine hydrochloride, add it to 100mL of absolute ethanol, stir at 400r / min for 20min, add 12mL of epichlorohydrin dropwise at 0.5mL / min into the mixture, and keep the temperature at 30°C Under a water bath, react for 4 hours, distill under reduced pressure to 40% of the volume of the original solution, and filter with suction to obtain a white needle-like solid; then weigh 60 g of the starch-based dodecyl glucoside pre...

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PUM

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Abstract

The invention discloses a preparation method of alkyl glycoside of an asymmetric Gemini structure, and belongs to the technical field of alkyl glycoside preparation. The preparation method comprises the following steps: taking cassava starch as a raw material to directly prepare starch-based lauryl glycoside, carrying out substitution and quaternization with hexadecyl dimethyl amine and epoxy chloropropane to synthesize the alkyl glucoside surfactant of the asymmetric Gemini structure. The alkyl glycoside of the asymmetric Gemini structure not only is as simple as common alkyl glycoside, but also has the advantage that neither effluent nor pollutants are discharged in the preparation process, so that environmental pollution is avoided. Moreover, due to high efficiency of the asymmetric Gemini structure, the alkyl glycoside of the asymmetric Gemini structure has excellent foam property and emulsifying property, has good wettability, and can be widely used in the biochemical industry, the food processing industry, the cosmetics industry and other industries.

Description

technical field [0001] The invention discloses a method for preparing an asymmetric Gemini-structured alkyl glycoside, belonging to the technical field of alkyl glycoside preparation. Background technique [0002] Alkyl glycoside (APG) is synthesized from natural fatty alcohol and glucose from renewable resources. It has excellent ecological and toxicological properties, excellent physical and chemical properties, and good compatibility. It has low surface tension and strong detergency. , the foam is rich and delicate, can be compounded with any type of surfactant, the synergistic effect is obvious, and it is non-toxic, harmless, non-irritating, and its biodegradability is better than any other type of surfactant. It is a new type of excellent performance Nonionic surfactants, which have the characteristics of ordinary nonionic and anionic surfactants, have high surface activity, good ecological safety and compatibility, and are also internationally recognized as the first c...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C11D1/66C08B31/12
CPCC08B31/125C11D1/662
Inventor 郭迎庆王龙薛蕾
Owner 郭迎庆