Spandex fiber and its preparation method, fabric
A technology of spandex fiber and fiber-forming polymer, which is applied in the fields of fiber chemical characteristics, textile and papermaking, single-component synthetic polymer rayon, etc., can solve the problems of high investment, difficulty in forming spinning dope, and affecting comfort
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[0029] The preparation method of the polyether type polyurethane segment in the present invention can adopt known polyurethane reaction technology. For example, the urethane prepolymer A having an isocyanate group at the end can be synthesized by reacting polyether diol and diisocyanate under the condition of excess diisocyanate. Preferably, a prepolymer A with an isocyanate group at the end can be synthesized by reacting an excess equivalent of diisocyanate with polytetramethylene ether glycol with a number average molecular weight of 500-5000; for example, 4,4'-diphenylmethane The molar ratio of diisocyanate to polytetramethylene ether glycol may be 1.5:1 to 2.0:1.
[0030] In traditional spandex preparation, the urethane prepolymer is generally further subjected to a chain extension reaction with a bifunctional amine to directly obtain a polyurethane urea polymer. Even if the spandex is further modified, it is carried out on the polyurethane urea polymer, for example, mixi...
Embodiment 1
[0058] Step 1: Preparation of Prepolymer C
[0059] 1) Mix polytetramethylene ether glycol with a number average molecular weight of 2000 and 4,4'-diphenylmethane diisocyanate, and react at 90°C for 100 minutes to obtain a polyurethane prepolymer A with isocyanate groups at the end, The molar ratio of 4,4'-diphenylmethane diisocyanate to polytetramethylene ether glycol is 1.70:1.
[0060] 2) After mixing polyethylene oxide glycol with a number average molecular weight of 1200 and 1,2-propanediol-3-sodium sulfonate evenly, mix it with 2,4'-diphenylmethane diisocyanate and 4, A mixture of 4'-diphenylmethane diisocyanate is mixed, wherein the mass ratio of 2,4'-diphenylmethane diisocyanate and 4,4'-diphenylmethane diisocyanate is 1:9, and the ratio of isocyanate group to hydroxyl group The molar ratio is 2.00:1. The above mixture was reacted at 90° C. for 120 minutes to obtain a polyurethane oligomer B having an isocyanate group at the end.
[0061] 3) Mix prepolymer A and oli...
Embodiment 2
[0072] Step 1: Preparation of Prepolymer C
[0073] 1) Mix raw materials polytetramethylene ether glycol with a number average molecular weight of 1800 and 4,4'-diphenylmethane diisocyanate, and react at 90°C for 100 minutes to obtain a polyurethane prepolymer A with an isocyanate group at the end, The molar ratio of 4,4'-diphenylmethane diisocyanate to polytetramethylene ether glycol is 1.70:1.
[0074] 2) After mixing polyethylene oxide glycol with a number average molecular weight of 1200 and 1,2-propanediol-3-sodium sulfonate evenly, mix it with 2,4'-diphenylmethane diisocyanate and 4, A mixture of 4'-diphenylmethane diisocyanate is mixed, wherein the mass ratio of 2,4'-diphenylmethane diisocyanate and 4,4'-diphenylmethane diisocyanate is 1:9, and the ratio of isocyanate group to hydroxyl group The molar ratio is 2.00:1. The above mixture was reacted at 90° C. for 120 minutes to obtain a polyurethane oligomer B having an isocyanate group at the end.
[0075] 3) Mix prep...
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