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Preparation and application of a hypochlorite intercalated layered composite metal hydroxide

A hypochlorite and composite metal technology, which is applied in the field of water treatment to achieve the effects of good ion exchange capacity, wide application range and high treatment sensitivity

Active Publication Date: 2020-06-02
TONGJI UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

What's more serious is that the combined pollution of arsenic and various organic pollutants has been detected in rivers and lakes used as drinking water sources in many areas of our country. Simultaneous removal of pollutants

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] A hypochlorite intercalated layered composite metal hydroxide for synergistically removing composite pollution in water, the preparation method of which comprises the following steps:

[0026] (1) Prepare 100ml of the first solution containing 150mmol L -1 Mg 2+ , 50mmol·L -1 Fe 3+ ; prepare another 100ml of the second solution containing 400mmol L -1 NaOH and 100mmol·L -1 Na 2 CO 3 ; Prepare another 20mmol·L -1 sodium hypochlorite solution.

[0027] (2) Add the above-mentioned configured first solution and second solution dropwise to a beaker containing 100ml of deionized water at the same time, stir vigorously during the dropwise addition, and control the pH value of the reaction process to remain at 9, and react The obtained slurry was aged at 60°C for 36 hours, and then solid-liquid separation was performed, and the obtained solid precipitate was washed with deionized water until the supernatant was neutral, then dried at 60°C, and calcined at 400°C , The o...

Embodiment 2

[0031] A hypochlorite intercalated layered composite metal hydroxide for synergistically removing composite pollution in water, the preparation method of which comprises the following steps:

[0032] (1) Prepare 100ml of the first solution containing 900mmol L -1 Mg 2+ , 285mmol·L -1 Fe 3+ and 15mmol·L -1 Ce 3+ , prepare another 100ml of the second solution, containing 4800mmol·L -1 NaOH and 1200mmol·L -1 Na 2 CO 3 , another preparation of 100mmol·L -1 sodium hypochlorite solution.

[0033](2) Add the above-mentioned configured first solution and the second solution dropwise to a beaker containing 100ml of deionized water at the same time, stir vigorously during the dropwise addition, and simultaneously control the pH value of the reaction process to remain at 10. The obtained slurry was aged at 70°C for 24 hours, and then solid-liquid separation was performed, and the obtained solid precipitate was washed with deionized water until the supernatant was neutral, then ...

Embodiment 3

[0037] A hypochlorite intercalated layered composite metal hydroxide for synergistically removing composite pollution in water, the preparation method of which comprises the following steps:

[0038] (1) Prepare 100ml of the first solution containing 300mmol L -1 Mg 2+ , 95mmol·L -1 Fe 3+ and 5mmol·L -1 Ce 3+ , prepare another 100ml of the second solution containing 800mmol·L -1 NaOH and 200mmol·L -1 Na 2 CO 3 , another preparation of 100mmol·L -1 sodium hypochlorite solution.

[0039] (2) Add the above-mentioned configured first solution and second solution dropwise to a beaker containing 100ml of deionized water at the same time, stir vigorously during the dropwise addition, and simultaneously control the pH value of the reaction process to remain at 11, and react The obtained slurry was aged at 80°C for 20 hours, and then solid-liquid separation was performed, and the obtained solid precipitate was washed with deionized water until the supernatant was neutral, the...

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PUM

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Abstract

The invention relates to a hypochlorous acid root-plugging layer laminar composite metal hydroxide for removing water pollutant, and a preparation method and an application. The method includes steps of mixing solution containing Mg2+, Fe3+, Ce3+ with sodium hydroxide and sodium carbonate solution in the de-ionized water; stirring the mixture; after aging, solid-fluid separation, drying and calcining, performing intercalation reaction in the pypocholoride solution; drying the acquired sediment, and acquiring the hypochlorous acid root-plugging layer laminar composite metal hydroxide. The material can be used for absorbing and removing arsenic in the water, absorb arsenic while release hypochlorite, thereby further oxidizing organic pollutant in the water and sterilizing germs. Compared with the prior art, the method compounds a new hypochlorous acid root-plugging layer laminar composite metal hydroxide; the material can be used for absorbing and removing arsenic in the water, absorb arsenic while release hypochlorite, thereby further oxidizing organic pollutant in the water and sterilizing germs cooperatively; therefore, the composite metal hydroxide is high in utilizing efficiency, and needs not to add oxidant, sterilizing agent and others additionally.

Description

technical field [0001] The invention relates to the field of water treatment, in particular to the preparation and application of a hypochlorite intercalated layered composite metal hydroxide. Background technique [0002] Arsenic is a toxic and carcinogenic element ubiquitous in nature. Arsenic pollution in drinking water sources is an environmental problem that has attracted global attention. At present, there are arsenic pollution problems in large areas in more than a dozen countries in the world. my country It is also one of the countries with serious arsenic pollution. The arsenic pollution in groundwater and rivers in some areas of my country is very serious. At present, the removal methods of arsenic in water include coagulation, coprecipitation, membrane separation, adsorption and so on. The adsorption method has been widely used in drinking water engineering due to its advantages of cost-effectiveness, high efficiency and convenient operation. At the same time, th...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/04B01J20/28B01J20/30A01N59/16A01N59/00A01N59/06A01P3/00A01P1/00B01J27/128C02F1/28
CPCA01N59/00A01N59/06A01N59/16B01J20/046B01J20/28033B01J27/128C02F1/281C02F2101/103A01N2300/00
Inventor 芦洪涛隋铭皓朱志良
Owner TONGJI UNIV