Method for rapidly absorbing heavy metal chromium ions in wastewater
A technology for chromium ions and heavy metals, applied in the field of rapid removal of heavy metal ions in wastewater, can solve the problems of difficult to achieve satisfactory results, secondary pollution, complicated operation, etc., and achieve the effect of easy industrial scale-up, high-dose adsorption, and simple operation
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Embodiment 1
[0024] The preparation of graphene microsphere adsorbent comprises the steps:
[0025] Ultrapure water was added to graphene oxide to prepare a graphene oxide solution with a mass concentration of 8 wt.%, and the solution was placed in an ultrasonic atomizer connected to a tube furnace with an ultrasonic frequency of 1.5 MHz. Make it atomized into aerosol droplets, and slowly pass through a tube furnace heated to 400°C under the drive of N2 and a filter vacuum pump, and collect it with a 0.22 um PTFE filter membrane at the end. Dry at room temperature for 8 hours to obtain the graphene microsphere adsorbent, and the particle size of the graphene microspheres prepared by the present invention is about 5 um.
Embodiment 2
[0027] The adsorption experiment of graphene microsphere adsorbent on chromium ion under different time, including the following steps
[0028] 10 mg of graphene microsphere adsorbent was accurately weighed with an electronic balance, and added to 20 mL of chromium ion solution with a concentration of 400 mg / L. Under the conditions of room temperature, 100 rpm and pH=6.0, adsorb for different times, and then centrifuge at 10000 rpm for 8 minutes,
[0029] And use the ultraviolet spectrophotometer to test the change of its absorbance before and after adsorption, and calculate the adsorption amount of the adsorbent at different times according to the following formula.
[0030] q(t)=(C0-Ct)V / m
[0031] In the formula, q(t) represents the adsorption amount (mg / g) at time t; C0 and Ct represent the chromium ion concentration (mg / L) in the initial solution respectively, and the chromium ion concentration (mg / L) in the solution at time t, And the chromium ion concentration (mg / L) ...
Embodiment 3
[0034] The test of adsorption isotherm comprises the following steps:
[0035] Accurately weigh 10 mg of graphene microsphere adsorbent with an electronic balance, and add it to 20 mL of chromium ion solution with a concentration range of 40-800 mg / L. Under the conditions of room temperature, 100 rpm and pH=6.0, adsorb for 120 min, and use a UV spectrophotometer to test the change of absorbance before and after adsorption, so as to calculate the concentration of residual chromium ions in each solution, draw the adsorption isotherm, and test The maximum adsorption capacity of graphene microspheres, see figure 2 . It can be seen from the figure that the adsorption capacity of the adsorbent increases with the increase of the concentration of chromium ions in the solution until the adsorption reaches equilibrium. When the concentration of chromium ions is low, the adsorption capacity of the adsorbent is less, which may be because at low concentrations, the adsorption sites on t...
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