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Method for reducing ethanol in polysulfide silane coupling agent

A technology of silane coupling agent and polysulfide, which is applied in the field of reducing ethanol content in silane coupling agent, can solve problems such as the influence of rubber comprehensive performance, improve safety, benefit health and environmental protection, and reduce ethanol content Effect

Inactive Publication Date: 2019-01-18
北京沃杰知识产权有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The technical problem to be solved by the present invention is to overcome the defect that the residual catalyst affects the comprehensive performance of rubber in the existing method for reducing ethanol in polysulfide silane, and then provides a method for reducing polysulfide silane coupling agent. ethanol method

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0024] The method for reducing ethanol in the polysulfide silane coupling agent provided by the present embodiment may further comprise the steps:

[0025] Preparation of composite alumina catalyst:

[0026] (1) Disperse the X-type molecular sieve into 0.1mol / L cerium nitrate aqueous solution to carry out ion exchange reaction at 75°C, filter after 7 hours of reaction, wherein the mass ratio of molecular sieve to metal cerium=1:25, collect the solid phase, The solid phase was dried at 60°C for 3 hours, and then calcined at 450°C for 2 hours to obtain a cerium-modified molecular sieve;

[0027] (2) Mix the cerium-modified molecular sieve prepared in step (1) with alumina dry rubber powder in a ratio of 1:0.2 in mass ratio, then add an appropriate amount of silica sol and starch to form a mixture, and extrude the mixture Shaped, dried at 90°C for 2 hours, and then calcined at 300°C for 5 hours to obtain a composite alumina catalyst.

[0028] Reduction of ethanol in polysulfide...

Embodiment 2

[0032] The method for reducing ethanol in the polysulfide silane coupling agent provided by the present embodiment may further comprise the steps:

[0033] Preparation of composite alumina catalyst:

[0034] (1) Disperse type A molecular sieve into 0.3 mol / L yttrium nitrate aqueous solution at 100°C for ion exchange reaction, filter after 10 hours of reaction, wherein the mass ratio of molecular sieve to metal yttrium=1:15, collect the solid phase, The solid phase was dried at 70°C for 2.5 hours, and then calcined at 350°C for 3 hours to obtain yttrium-modified molecular sieves;

[0035] (2) Mix the yttrium-modified molecular sieve prepared in step (1) with alumina dry rubber powder in a ratio of 1:0.6 in mass ratio, then add an appropriate amount of silica sol and starch to form a mixture, and extrude the mixture Shaped, dried at 80°C for 3 hours, and then calcined at 400°C for 4 hours to obtain a composite alumina catalyst.

[0036] Reduction of ethanol in polysulfide sila...

Embodiment 3

[0040] The method for reducing ethanol in the polysulfide silane coupling agent provided by the present embodiment may further comprise the steps:

[0041] Preparation of composite alumina catalyst:

[0042] (1) Disperse the Y-type molecular sieve into 0.15mol / L lanthanum nitrate aqueous solution to carry out ion exchange reaction at 90°C, filter after reacting for 8h, wherein the mass ratio of molecular sieve to metal lanthanum=1:18, collect the solid phase, The solid phase was dried at 70°C for 3 hours, and then calcined at 400°C for 4 hours to obtain a lanthanum-modified molecular sieve;

[0043] (2) Mix the lanthanum-modified molecular sieve prepared in step (1) with the dry rubber powder of alumina in a mass ratio of 1:0.3, then add an appropriate amount of silica sol and starch to form a mixture, and extrude the mixture Shaped, dried at 75°C for 2 hours, and then calcined at 350°C for 5 hours to obtain a composite alumina catalyst.

[0044] Reduction of ethanol in poly...

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PUM

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Abstract

The invention provides a method for reducing ethanol in a polysulfide silane coupling agent. The method comprises the steps of mixing the polysulfide silane coupling agent, dihydric alcohol, ethanol and a compound alumina catalyst for reaction so as to evaporate ethanol out of the polysulfide silane coupling agent, after the reaction is finished, sequentially carrying out atmospheric distillationand reduced pressure distillation until no fraction flows out so as to evaporate residual ethanol and unreacted dihydric alcohol out of the polysulfide silane coupling agent, cooling, and filtering, so as to obtain the polysulfide silane coupling agent free of ethanol. The method has the beneficial effects that on one hand, the reaction between the polysulfide silane coupling agent and dihydric alcohol can be promoted through the compound alumina catalyst, so that a large number of ethanol in the polysulfide silane coupling agent can be replaced, and the content of ethanol in the polysulfide silane coupling agent can be reduced; and meanwhile, the compound alumina catalyst is a solid catalyst, so that the solid catalyst only needs to be filtered in the after-treatment process.

Description

technical field [0001] The present invention relates to the method for reducing ethanol content in silane coupling agent, be specifically related to a kind of method for reducing ethanol in polysulfide silane coupling agent. Background technique [0002] Polysulfide silane coupling agents are widely used in sealing compounds, cast metal parts, pigments, protective coatings, adhesives, asphalt mixtures and rubber additives. It can improve the compatibility between rubber and fillers (such as carbon black, white carbon black), improve the comprehensive performance of rubber products, and is a commonly used rubber additive. Taking automobile tires as an example, the addition of polysulfide silane coupling agents can significantly improve the performance of tires such as wet skid resistance, wear resistance and heat generation. At present, in the automobile tire industry, the most widely used polysulfide silane coupling agent is bis-[3-(triethoxysilyl)propyl]-tetrasulfide, whic...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C07F7/18C07F7/20
CPCC07F7/20
Inventor 付佩学刘超李建军
Owner 北京沃杰知识产权有限公司