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Method for synthesizing acetone ketal glycerinum acetate from glycerinum

A technology of acetone acetal acetate and acetone acetal is applied in the field of production technology of acetone acetal acetate, can solve the problems of increasing atomization, reducing fuel viscosity, etc., and achieves the advantages of less equipment corrosion, environmental protection and high yield. Effect

Active Publication Date: 2019-12-03
山东衡兴新材料科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Acetone glycidyl acetate can be used as a biofuel and biodiesel additive, which can significantly increase the fuel flash point. In addition, it can significantly reduce the fuel viscosity, resulting in increased atomization and more complete combustion. It is in line with the development direction of green chemical industry and has a strong Industrial application background, but there is no relevant literature report

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] 1) Add 2 mol of glycerol, a by-product of biodiesel (accounting for about 10% of the total mass of biodiesel), to the condensation reactor after pretreatment, deodorization, decolorization, and rectification to a purity of 98%, and then press glycerol: acetone = 1 : 2 (ratio of substances, the same below) Add acetone to the condensation kettle, add acidic ion exchange resin HND-580 according to 1% of the mass of glycerin, and stir at 40°C for 4.5h for condensation reaction; after the condensation reaction is completed, transfer the product to the extraction kettle, cooled to room temperature, and extracted three times with an equal volume of butyl ether. The extract was heated to 75°C by a heater and entered into a rectification tower. Under the condition of vacuum degree of 0.099-0.1, collect the distillate at 80-83°C, which is acetonide;

[0024] 2) Add 1 mol of acetonide to the reaction / azeotropic distillation device, and add acetone glycerol with a mass of 0.1 % KO...

Embodiment 2

[0026] 1) Add 2 mol of glycerin, a by-product of biodiesel (accounting for about 10% of the total mass of biodiesel), to the condensation reactor after pretreatment, deodorization, decolorization, and rectification, and then press glycerol: acetone = 1:3 Add acetone, add acidic ion exchange resin HND-580 according to 3% of glycerin mass, and stir and react at 50°C for 3h; The second time, the extract is heated by a heater to 75°C and enters the rectification tower, acetone is evaporated at normal pressure, butyl ether is evaporated under reduced pressure for recycling, and then the fraction at 80-83°C is collected under the condition of vacuum degree of 0.099-0.1MPa , which is acetone glycalol;

[0027] 2) Add 1 mol of acetonide to the reaction / azeotropic distillation device, and add acetone glyceride mass 0.2% solid K according to acetone glycerol: propyl acetate = 1:10 (mass ratio) 2 CO 3 , reacted at 100°C, and refluxed for 8 hours, until the content of propanol in the to...

Embodiment 3

[0029] 1) Add 2 mol of glycerin, a by-product of biodiesel (accounting for about 10% of the total mass of biodiesel), to the condensation reactor after pretreatment, deodorization, decolorization, and rectification, and then add glycerin: acetone = 1:5 Add acetone, add acidic ion exchange resin HND-580 according to 5% glycerin mass, and stir and react at 60°C for 1 h; after the condensation reaction is completed, transfer the product to an extraction kettle, cool to room temperature, and extract with 3 times the volume of butyl ether Three times, the extract was heated by a heater to 75°C and entered the rectification tower, acetone was steamed under normal pressure, butyl ether and acetonide were evaporated under reduced pressure, and the 80-83°C was collected under the condition of vacuum degree of 0.099-0.1MPa. The distillate is acetonide;

[0030] 2) Add acetonide to the reaction / azeotropic distillation device, add acetone mass 0.2% CH according to acetone: propyl acetate ...

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PUM

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Abstract

The invention discloses a method for synthesizing acetone ketal glycerinum acetate from glycerinum. The method comprises the following steps: firstly, putting acetone and a biodiesel byproduct, namelyglycerinum, into a condensation kettle, performing a condensation reaction in the presence of a catalyst A, and performing extraction and distillation after the reaction so as to obtain acetone ketalglycerinum; putting the acetone ketal glycerinum into a reaction / azeotropic distillation device, performing an ester exchange reaction with acetate in the presence of a catalyst B, and performing aftertreatment, so as to obtain a target product, namely the acetone ketal glycerinum acetate. Through condensation and ester exchange reactions, the biodiesel byproduct, namely the glycerinum, is converted into the acetone ketal glycerinum acetate which can be used as a fuel additive, separation is simple, the yield is high, the preparation process is simple, the catalyst is small in equipment corrosion, environment pollution caused by glycerinum wastes can be avoided, the environment can be protected, meanwhile, additional values of products can be increased, and development of the biodiesel industry can be facilitated.

Description

technical field [0001] The invention belongs to the technical field of energy recycling, in particular to a production process of acetone glycidyl acetate. Background technique [0002] Glycerin is a by-product of the biodiesel production process. It has low calorific value, is difficult to burn, and is insoluble in non-polar compounds such as fuels. Therefore, it is difficult to be utilized, and manufacturers usually dispose of it as waste. This not only caused huge environmental pollution, but also caused losses to the profits of manufacturers. The conversion of glycerol to acetone glycidyl acetate is one way to solve the problem of excess glycerol. Acetone glycidyl acetate can be used as a biofuel and biodiesel additive, which can significantly increase the fuel flash point. In addition, it can significantly reduce the fuel viscosity, resulting in increased atomization and more complete combustion. It is in line with the development direction of green chemical industry a...

Claims

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Application Information

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IPC IPC(8): C07D317/24
CPCC07D317/24
Inventor 任杰熊俊豪王恒秀
Owner 山东衡兴新材料科技有限公司