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A kind of preparation method of multi-metal composite oxygen carrier

A technology of oxygen carrier and multi-metal, which is applied in the field of preparation of multi-metal composite oxygen carrier to achieve high conversion rate of ethane or propane, increase conversion rate and prolong reaction time

Active Publication Date: 2021-12-28
QINGDAO UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The purpose of the present invention is to overcome the shortcomings of the prior art, aiming at the defect that lattice oxygen transforms to adsorbed oxygen in the reaction process, it is designed to provide a method for preparing a multi-metal composite oxygen carrier, which can effectively control the crystal lattice oxygen release, thereby inhibiting its direction conversion

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0035] The specific process of preparing multi-metal composite oxygen carrier in this embodiment is as follows:

[0036] (1) Preparation of alumina carrier: screen 500g of alumina particles with a particle size of 80-800 μm, add 3-6g of scallop powder, mix well, add 100ml of 2% nitric acid aqueous solution dropwise, and place in a 100°C refrigerator after fully mixing After drying in an oven for 48 hours, calcining in a muffle furnace at 500-600°C to obtain alumina carrier particles;

[0037] (2) First mix the binder and clay according to the mass ratio of 2:8 and dissolve them in deionized water to form a slurry with a mass fraction of 50%, and then fully disperse the alumina carrier prepared in step (1) In the prepared slurry, the slurry is then spray-dried, and sieved to obtain particles with a particle size of 80-600 μm;

[0038] (3) getting mass fraction is 99% ferric nitrate nonahydrate (Fe(NO 3 ) 3 9H 2 O) 200g and 99.9% cerium nitrate hexahydrate (Ce(NO 3 ) 3 ·6H...

Embodiment 2

[0051] The specific process of preparing multi-metal composite oxygen carrier in this embodiment is as follows:

[0052] (1) Preparation of alumina carrier: screen 500g of alumina particles with a particle size of 80-800 μm, add 3-6g of scallop powder, mix well, add 100ml of 2% nitric acid aqueous solution dropwise, and place in a 100°C refrigerator after fully mixing After drying in an oven for 48 hours, calcining in a muffle furnace at 500-600°C to obtain alumina carrier particles;

[0053] (2) First mix the binder and clay according to the mass ratio of 4:6 and dissolve them in deionized water to form a slurry with a mass fraction of 60%, and then fully disperse the alumina carrier prepared in step (1) In the prepared slurry, the slurry is then spray-dried, and sieved to obtain particles with a particle size of 80-600 μm;

[0054] (3) getting mass fraction is 99% ferric nitrate nonahydrate (Fe(NO 3 ) 3 9H 2 O) 100g and 99.5% cerium nitrate hexahydrate (Ce(NO 3 ) 3 ·6H...

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Abstract

The invention belongs to the technical field of oxygen carrier preparation, and relates to a preparation method of a multi-metal composite oxygen carrier. A weakly oxidizing oxygen carrier is selected for dehydrogenation reaction, and the prepared oxygen carrier contains Fe 2 o 3 , CeO 2 and BaO, three oxides can tune the Al 2 o 3 The acidic sites on the surface of the carrier, at the same time, the three metal elements can attract lattice oxygen to the surface of the oxygen carrier, and react with the hydrogen removed from the ethane or propane on the active site to form water, which promotes the positive progress of the reaction, thus The selectivity of ethylene or propylene is improved; compared with the pure Mn-based oxygen carrier, the Fe-Ce composite oxygen carrier increases the oxygen carrying capacity of the oxygen carrier, thereby prolonging the reaction time between the oxygen carrier and the alkane.

Description

Technical field: [0001] The invention belongs to the technical field of oxygen carrier preparation, and relates to a preparation method of a multi-metal composite oxygen carrier, which can be used for the production of ethylene by chemical chain dehydrogenation of ethane and the production of propylene by chemical chain dehydrogenation of propane. Background technique: [0002] At present, most of the low-carbon alkanes produced in China are directly used as fuel, and their utilization value needs to be improved, especially the supply of ethylene is still in short supply. Therefore, the study of dehydrogenation of light alkanes to olefins can realize the effective utilization of petroleum cracking gas. In 2015, the domestic demand for ethylene is expected to be over 30.14 million tons, while the annual domestic ethylene output in 2015 was only 22.45 million tons, which is far below the demand. In order to meet the huge demand for ethylene, ethane production has been widely c...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/83B01J37/08B01J35/10C07C5/333C07C11/04C07C11/06
CPCB01J23/83B01J23/002B01J37/0018C07C5/3332B01J2523/00B01J35/397B01J35/635B01J35/615C07C11/04C07C11/06B01J2523/25B01J2523/3712B01J2523/842Y02P20/52
Inventor 郭庆杰左成吴曼刘永卓安阳袁思杰
Owner QINGDAO UNIV OF SCI & TECH