A kind of graphene oxide graft modified oleic acid soap, concentrated solution for hydraulic support, preparation method and application
A technology of graft modification and hydraulic support, which is applied in the petroleum industry, additives, lubricating compositions, etc., to achieve the effects of avoiding leakage, good sealing and material compatibility, and broad application prospects
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Embodiment 1
[0043] 1. Preparation of Graphene Oxide Grafted Modified Oleic Acid Soap
[0044] (1) Add 0.5g of graphene oxide, 85mL of thionyl chloride and 4mL of N,N-dimethylformamide into a three-necked flask, react at 68°C for 24h, filter, and dry at 70°C for 24h to obtain a carboxyl group Activated graphene oxide;
[0045] (2) Add 0.008g of graphene oxide with activated carboxyl groups to 10mL N, N-dimethylformamide, ultrasonically disperse for 10min, add to a three-necked flask containing 60g of triethanolamine, and stir at 200rpm, 95 ℃ for 4.5 hours, the temperature was raised to 128 ℃, 20 g of oleic acid was added, and the reaction was continued for 2 hours to obtain the graphene oxide grafted modified oleic acid soap.
[0046] 2. Preparation of Castor Potassium Soap
[0047] Add 22g of castor oil, 13.5g of potassium hydroxide and 30g of water into a three-necked flask, mix well, and react at 78°C for 4h under the stirring condition of 200rpm to obtain the castor potassium soap, w...
Embodiment 2
[0055] 1. Preparation of Graphene Oxide Grafted Modified Oleic Acid Soap
[0056] (1) Add 0.6g of graphene oxide, 95mL of thionyl chloride and 6mL of N,N-dimethylformamide into a three-necked flask, react at 75°C for 23h, filter, and dry at 70°C for 24h to obtain a carboxyl group Activated graphene oxide;
[0057] (2) Add 0.010 g of graphene oxide with activated carboxyl groups to 16 mL of N,N-dimethylformamide, ultrasonically disperse it for 10 min, add it to a three-necked flask containing 40 g of triethanolamine, and stir at 200 rpm for 105 ℃ for 3.5 hours, the temperature was raised to 125 ℃, 30 g of oleic acid was added, and the reaction was continued for 3 hours to obtain the graphene oxide grafted modified oleic acid soap.
[0058] 2. Preparation of Castor Potassium Soap
[0059] Add 10g of castor oil, 10g of potassium hydroxide and 20g of water into a three-necked flask, mix well, and react at 80°C for 3.5h under the stirring condition of 200rpm to obtain the castor ...
Embodiment 3
[0067] 1. Preparation of Graphene Oxide Grafted Modified Oleic Acid Soap
[0068] (1) Add 0.8g of graphene oxide, 90mL of thionyl chloride and 8mL of N,N-dimethylformamide into a three-necked flask, react at 65°C for 25h, filter, and dry at 70°C for 24h to obtain a carboxyl group Activated graphene oxide;
[0069] (2) Add 0.012g of graphene oxide with activated carboxyl groups to 20mL N, N-dimethylformamide, ultrasonically disperse for 10min, add to a three-necked flask containing 55g of triethanolamine, and stir at 200rpm, 100 ℃ for 4 hours, the temperature was raised to 135 ℃, 10 g of oleic acid was added, and the reaction was continued for 2 hours to obtain the graphene oxide grafted modified oleic acid soap.
[0070] 2. Preparation of Castor Potassium Soap
[0071] Add 18g of castor oil, 8g of potassium hydroxide and 30g of water into a three-necked flask, mix well, and react at 70°C for 4.5h under the stirring condition of 200rpm to obtain the castor potassium soap, whi...
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