Adhesive for repeatedly foldable device, adhesive sheet, repeatedly foldable laminate member and repeatedly foldable device
A technology of repeated bending and adhesive layer, applied in the direction of adhesives, adhesive types, electric solid devices, etc., can solve the problems of floating and peeling, and achieve the effect of excellent bending resistance and not easy to float or peel
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preparation example Construction
[0074] (2) Preparation of Adhesive Composition P
[0075] The adhesive composition P can be prepared by preparing the (meth)acrylate polymer (A), mixing the obtained (meth)acrylate polymer (A) with the crosslinking agent (B), and simultaneously Add additives as needed.
[0076] The (meth)acrylate polymer (A) can be produced by polymerizing a mixture of monomers constituting a polymer by a normal radical polymerization method. The polymerization of the (meth)acrylate polymer (A) is preferably performed by a solution polymerization method using a polymerization initiator as needed. By polymerizing the (meth)acrylate polymer (A) by the solution polymerization method, it becomes easy to increase the molecular weight of the obtained polymer and to adjust the molecular weight distribution, and it is possible to further reduce the production of low molecular weight bodies. Therefore, even when the gel fraction is small and the degree of crosslinking is slowed down, the adhesive is ...
manufacture example
[0109] As one production example of the adhesive sheet 1, the case where the said adhesive composition P is used is demonstrated. A coating solution of the adhesive composition P is coated on the peeling surface of a release sheet 12a (or 12b), and heat-treated to form a coating layer by thermally crosslinking the adhesive composition P. The peeling surface of another peeling sheet 12b (or 12a) is superimposed on it. When the aging period is required, the coating layer becomes the adhesive layer 11 by setting the aging period, and when the aging period is unnecessary, the coating layer becomes the adhesive layer 11 directly. Thus, the above-mentioned adhesive sheet 1 was obtained. The conditions of heat treatment and aging are as above.
[0110] As another production example of the adhesive sheet 1, a coating solution of the adhesive composition P is applied to the release surface of one release sheet 12a, and heat-treated to thermally crosslink the adhesive composition P to...
Embodiment
[0134] Hereinafter, although an Example etc. demonstrate this invention more concretely, the scope of the present invention is not limited by these Examples etc.
[0135] 1. Preparation of (meth)acrylate polymer (A)
[0136] The n-butyl acrylate of 54 mass parts, the 2-ethylhexyl acrylate of 45 mass parts and the 4-hydroxybutyl acrylate of 1 mass part are copolymerized by solution polymerization, thereby prepare (meth)acrylic acid ester polymer (A ). As a result of measuring the molecular weight of this (meth)acrylate polymer (A) by the method mentioned later, the weight average molecular weight (Mw) was 800,000.
[0137] 2. Preparation of Adhesive Composition
[0138] 100 parts by mass (value in terms of solid content; hereinafter the same) of the (meth)acrylate polymer (A) obtained in the above step 1, 0.25 parts by mass of trimethylolpropane modified as a crosslinking agent (B) Xylylene diisocyanate (XDI; manufactured by Soken Chemical & Engineering Co., Ltd., product na...
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