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A production system and production method for reducing the content of sodium ions and sulfate ions in the precursor of positive electrode materials

A sulfate ion and production system technology, applied in the direction of positive electrodes, battery electrodes, active material electrodes, etc., can solve the problems of high Na impurity content and insignificant effect, achieve simple production system and process, reduce chemical adsorption amount, The effect of reducing the content

Active Publication Date: 2021-10-29
ZHUJI PAWA NEW ENERGY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This patent reduces the S impurity content by optimizing the washing process, but the effect is not significant, and there is a high risk of Na impurity content

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0035] Step (1), add half a kettle of hot pure water at 60°C to the 26m³ batching kettle, add 1678.1Kg of nickel sulfate, 726.1Kg of cobalt sulfate, and 848.5Kg of manganese sulfate, stir for 3 hours and then add hot pure water to the batching kettle Set the position of the volume plate and stir for 1 hour to obtain a mixed salt solution with a concentration of 120g / L, and the molar ratio of nickel, cobalt and manganese is 5:2:3;

[0036] Step (2), set the stirring speed of the reactor to 220r / min, add hot water at 60°C to the full kettle, set the temperature of the reactor to 65°C, control the temperature of the reactor at 65°C during the process, add ammonia water, and test the reaction by titration Ammonia concentration in the kettle, stop adding ammonia water when the ammonia concentration reaches 7.8g / L, add sodium hydroxide solution, control the pH value, stop adding alkali when the measured pH value reaches 10.8;

[0037] Step (3), feed the mixed salt solution at a flow...

Embodiment 2

[0048] Step (1), add half a pot of 70°C hot pure water to the 26m³ batching kettle, add 1678.1Kg of nickel sulfate, 726.1Kg of cobalt sulfate, and 848.5Kg of manganese sulfate, stir for 3 hours and then add hot pure water to the batching kettle Set the position of the volume plate and stir for 1 hour to obtain a mixed solution with a concentration of 120g / L and a nickel-cobalt-manganese ratio of 5:2:3;

[0049] Step (2), set the stirring speed of the reactor to 220r / min, add hot water at 70°C to the full kettle, set the temperature of the reactor to 70°C, control the temperature of the reactor at 70°C during the process, add ammonia water, and test the reaction by titration Ammonia concentration in the kettle, stop adding ammonia water when the ammonia concentration reaches 8.0g / L, add sodium hydroxide solution, control the pH value, stop adding alkali when the measured pH value reaches 11.0;

[0050] Step (3), feed the mixed salt solution at a flow rate of 320L / h, and start f...

Embodiment 3

[0061] Step (1), add half a pot of hot pure water at 65°C to the 26m³ batching kettle, add 1678.1Kg of nickel sulfate, 726.1Kg of cobalt sulfate, and 848.5Kg of manganese sulfate, stir for 3 hours and add hot pure water again to reach the batching kettle Set the position of the volume plate and stir for 1 hour to obtain a mixed solution with a concentration of 120g / L and a nickel-cobalt-manganese ratio of 5:2:3;

[0062] Step (2), set the stirring speed of the reactor to 220r / min, add hot water at 65°C to the full kettle, set the temperature of the reactor to 65°C, control the temperature of the reactor at 65°C during the process, add ammonia water, and test the reaction by titration Ammonia concentration in the kettle, stop adding ammonia water when the ammonia concentration reaches 8.5g / L, add sodium hydroxide solution, control the pH value, stop adding alkali when the measured pH value reaches 11.2;

[0063] Step (3), feed the mixed salt solution at a flow rate of 350L / h, a...

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Abstract

The invention belongs to the field of lithium ion battery materials, and in particular relates to a production system and a production method for reducing sodium ions and sulfate ions, the precursors of positive electrode materials, for industrialized production. Through the circulation of materials between the reactor, overflow tank and precision filter, the solid content of the precursor precipitation reaction process is increased, the force between particles is increased, the compactness of primary particles is improved, and sodium ions and sulfate ions are reduced. The amount of physical adsorption; by reducing the content of free nickel in the reaction process, reduce the amount of chemical adsorption of sodium ions and sulfate ions. After the precipitation reaction, through the storage tank and thickener, the solid content of the material before washing is increased, and the physical adsorption of sodium ions and sulfate ions is reduced through the force between particles. The production system and method of the present invention greatly reduce the Na content of the positive electrode material precursor. + and SO 4 2‑ content.

Description

technical field [0001] The invention relates to the field of lithium ion battery materials, in particular to a production system and a production method for reducing the content of sodium ions and sulfate ions in a positive electrode material precursor. Background technique [0002] The new energy industry has developed rapidly due to its environmental protection and recycling. With the development of the new energy industry, the technology of new energy vehicles is also improving. Countries have also announced plans for new energy vehicles to gradually replace fuel vehicles. As the most environmentally friendly vehicle in the future, its safety performance and service life have become crucial performance indicators. [0003] Cathode materials account for more than 40% of the overall battery cost. The ternary cathode material is currently the most competitive material, with advantages such as high capacity, high cycle performance, and high safety performance. The physical ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01M4/505H01M4/525H01M10/0525
CPCH01M4/505H01M4/525H01M10/0525H01M2004/028Y02E60/10
Inventor 张宝王振宇
Owner ZHUJI PAWA NEW ENERGY