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A kind of preparation method of carbon fluoride modified iron trifluoride cathode material

A technology of ferric trifluoride and positive electrode materials, applied in the direction of positive electrodes, battery electrodes, active material electrodes, etc., can solve the problems of being unable to use and the performance of FeF3 not meeting the requirements, etc., and achieve extended working time and good uniform mixing effect , the effect of prolonging the holding time

Active Publication Date: 2022-07-12
GUIZHOU MEILING POWER SUPPLY CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] At present, FeF sold on the market 3 The performance does not meet the requirements and cannot be used
However, there are few reports on the preparation technology of ultra-high electrode potential cathode materials.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] A preparation method of a carbon fluoride modified iron trifluoride positive electrode material, comprising the following steps:

[0028] (1) adding the carbon fiber material to absolute ethanol, stirring for 1 h to obtain a uniform mixed solution;

[0029] (2) adding Fe powder passing through a 200-mesh sieve into the mixed solution, stirring for 1.5h to obtain a uniform mixture solution;

[0030] (3) heating the mixture solution to 50°C, continue stirring until a paste is obtained;

[0031] (4) Place the paste in a high-energy ball mill for high-energy ball milling, the rotational speed is 3000 r / min, and the high-energy ball milling time is 2 minutes, then stop running, cool for 20 minutes, run the high-energy ball mill again, repeat this step, and the total high-energy ball milling time reaches 2h, The mixed slurry is obtained; the high-energy ball mill uses a high-energy ball mill cup, and zirconia balls are added during ball milling;

[0032] (5) drying the mixe...

Embodiment 2

[0036] A preparation method of a carbon fluoride modified iron trifluoride positive electrode material, comprising the following steps:

[0037] (1) adding the carbon fiber material to acetone, stirring for 1.5h, to obtain a uniform mixed solution;

[0038] (2) adding Fe powder passing through 300 mesh sieves to the mixed solution, stirring for 1h to obtain a uniform mixture solution;

[0039] (3) heating the mixture solution to 60°C, and continuing to stir until a paste is obtained;

[0040] (4) Put the paste in a high-energy ball mill for high-energy ball milling, the rotational speed is 5000r / min, the high-energy ball milling time is 1min, then stop running, cool for 15min, run the high-energy ball mill again, repeat this step, the total time of high-energy ball milling reaches 1.5h , to obtain a mixed slurry; the high-energy ball mill uses a high-energy ball mill cup, and zirconia balls are added during ball milling;

[0041] (5) drying the mixed slurry at a temperature ...

Embodiment 3

[0045] A preparation method of a carbon fluoride modified iron trifluoride positive electrode material, comprising the following steps:

[0046] (1) adding the carbon fiber material to the dispersing agent, stirring for 2h to obtain a uniform mixed solution, the dispersing agent includes acetone and absolute ethanol, and the weight ratio of acetone and absolute ethanol is 1:1;

[0047] (2) adding Fe powder passing through a 250 mesh sieve into the mixed solution, stirring for 2h to obtain a uniform mixture solution;

[0048] (3) heating the mixture solution to 70°C, and continue stirring until a paste is obtained;

[0049] (4) Place the paste in a high-energy ball mill for high-energy ball milling, the rotational speed is 8000r / min, the high-energy ball milling time is 30s, then stop running, cool for 15min, run the high-energy ball mill again, repeat this step, the total high-energy ball milling time reaches 1h, The mixed slurry is obtained; the high-energy ball mill uses a hi...

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PUM

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Abstract

This scheme discloses a preparation method of a carbon fluoride modified iron trifluoride positive electrode material in the technical field of thermal battery materials. The Fe powder is added to the mixed solution and stirred to obtain a mixed solution; (3) the mixed solution is heated to 50°C to 70°C, and the stirring is continued until a paste is obtained; (4) the paste is subjected to high-energy ball milling to obtain a mixed paste (5) drying the mixed slurry at a temperature of 60-70 ℃, then cooling to normal temperature, and grinding the cooled mixed sauce to obtain Fe powder covered by carbon fiber; (6) wrapping the carbon fiber The coated Fe powder is fluorinated, cooled and ground to obtain a carbon fluoride modified iron trifluoride cathode material. FeF for this application 3 The positive electrode material can effectively prolong the working time of the battery, improve the working voltage of the single cell of the thermal battery, and then improve the specific characteristics of the thermal battery.

Description

technical field [0001] The invention belongs to the technical field of thermal battery materials, and particularly relates to a preparation method of a carbon fluoride modified iron trifluoride positive electrode material. Background technique [0002] The thermal battery is a thermally activated reserve battery. It is a disposable reserve battery activated by melting salt as an electrolyte and using a heat source to melt it. The internal temperature during operation is 450°C to 550°C. Due to the small internal resistance of the thermal battery, high specific energy and specific power, wide use environment temperature, long storage time, rapid and reliable activation, compact structure, no directionality during use and not affected by installation orientation, good mechanical properties, It does not need maintenance and other advantages. It is favored by the military as soon as it comes out, and it has developed into an ideal power source for modern weapons and emergency sys...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01M4/62H01M4/58H01M6/36
CPCH01M4/582H01M4/628H01M6/36H01M2004/028H01M2004/021Y02E60/10
Inventor 王京亮张红梅朱艳丽冉岭李美玉姚利潘志鹏刘方吴启兵
Owner GUIZHOU MEILING POWER SUPPLY CO LTD