Polymer dispersion liquid, preparation method thereof, polymer composite membrane and application of polymer composite membrane
A polymer dispersion and polymer technology, which is applied in the field of polymer material preparation, can solve the problems of high difficulty, many limitations of film forming process, low solid content and viscosity, etc., to improve mechanical properties, increase solid content, reduce Df and Effect of thermal expansion coefficient
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preparation example Construction
[0039] The present invention also provides a kind of preparation method of polymer dispersion liquid, comprises the following steps:
[0040] The first step is to synthesize polyamic acid solution.
[0041] Wherein, the polyamic acid is formed by polymerizing two kinds of diamine monomers and two kinds of dianhydride monomers, and the two kinds of diamine monomers and the two kinds of dianhydride monomers contain liquid crystal structure and flexible structure respectively. .
[0042] In this embodiment, diamine monomers containing liquid crystal structures include but are not limited to p-aminophenyl p-aminobenzoate (APAB), 1,4-bis(4-aminophenoxy)benzene (ABHQ) and p-aminophenylene One or more of bis-p-aminophenyl formate (BPTP). Diamine monomers with flexible structures include but are not limited to 4,4'-diaminodiphenyl ether (ODA), 2,2'-bis[4-(4-aminophenoxyphenyl)]propane (BAPP) One or more of 1,3-bis(4'-aminophenoxy)benzene (TPE-R) and 1,3-bis(3-aminophenoxy)benzene (...
Synthetic example 1
[0076] Add NMP (243.8g) and TPE-M (0.1mol, 29.23g) into a 500mL reaction bottle respectively, and after stirring until dissolved, add BPADA (0.1mol, 52.05g) and stir for 48 hours to complete the configuration of the polyamide acid solution.
Synthetic example 2
[0078] Add NMP (205.97g) and APAB (0.1mol, 22.83g) into a 500mL reaction bottle respectively, after stirring until dissolved, then add TAHQ (0.1mol, 45.83g) and stir for 48 hours to complete the configuration of the polyamic acid solution .
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